Stepped-Type Photoacoustic Resonator for Simultaneous Dual-Gas Detection

A stepped-type resonator-based photoacoustic (PA) sensor is proposed for simultaneous dual-gas detection. The sensor employs a dual-resonance architecture, with a stepped resonant tube capable of acoustic amplification at two different frequencies. An optimized design of the PA resonator response is conducted using finite element analysis. When the amplitudes of the two resonance peaks are high and the relative signal strength is also high, the simulated values of the two resonance frequencies are 2370 and 4220 Hz, respectively. A dual-channel synchronous digital lock-in amplifier is employed to achieve simultaneous detection in the two channels. Two lasers for methane and acetylene detection are modulated simultaneously, with the modulation frequencies set to half of these two resonant frequencies. The crosstalk evaluation results show that the signal crosstalk between the dual-gas detection channels is -125.26 dB, and the frequency crosstalk is -129.70 dB. Under a 1-s integration time, the minimum detection limits are 25.2 ppb for C<sub>2</sub>H<sub>2</sub> and 51.5 ppb for CH<sub>4</sub>, corresponding to normalized noise-equivalent absorption coefficients (NNEAs) of 1.62 × 10<sup>-9</sup> Wcm<sup>- 1</sup> Hz<sup>- 1/2</sup> and 9.98 × 10<sup>-10</sup> Wcm<sup>- 1</sup> Hz<sup>- 1/2</sup>, respectively.

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Publication Details

Journal
Analytical Chemistry
Published
2026-01-02
DOI
https://doi.org/10.1021/acs.analchem.5c05876
Citations
4
Primary Topic
Spectroscopy and Laser Applications
Type
article
Field-Weighted Citation Impact
65.05
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article

Stepped-Type Photoacoustic Resonator for Simultaneous Dual-Gas Detection

Bingyu Mo, Hongchao Qi, Jingya Zhang, Chun Sun et al.
4 citations
Analytical Chemistry
Spectroscopy and Laser Applications
65.05
article

Stepped-Type Photoacoustic Resonator for Simultaneous Dual-Gas Detection

Bingyu Mo, Hongchao Qi, Jingya Zhang, Chun Sun, Heng Wang, Ke Chen, Tianhe Yang
article en
4 citations

Abstract

A stepped-type resonator-based photoacoustic (PA) sensor is proposed for simultaneous dual-gas detection. The sensor employs a dual-resonance architecture, with a stepped resonant tube capable of acoustic amplification at two different frequencies. An optimized design of the PA resonator response is conducted using finite element analysis. When the amplitudes of the two resonance peaks are high and the relative signal strength is also high, the simulated values of the two resonance frequencies are 2370 and 4220 Hz, respectively. A dual-channel synchronous digital lock-in amplifier is employed to achieve simultaneous detection in the two channels. Two lasers for methane and acetylene detection are modulated simultaneously, with the modulation frequencies set to half of these two resonant frequencies. The crosstalk evaluation results show that the signal crosstalk between the dual-gas detection channels is -125.26 dB, and the frequency crosstalk is -129.70 dB. Under a 1-s integration time, the minimum detection limits are 25.2 ppb for C<sub>2</sub>H<sub>2</sub> and 51.5 ppb for CH<sub>4</sub>, corresponding to normalized noise-equivalent absorption coefficients (NNEAs) of 1.62 × 10<sup>-9</sup> Wcm<sup>- 1</sup> Hz<sup>- 1/2</sup> and 9.98 × 10<sup>-10</sup> Wcm<sup>- 1</sup> Hz<sup>- 1/2</sup>, respectively.

Analytical ChemistryVol. 98(1)
Jiangnan University (CN), Electric Power Research Institute (US), Dalian University of Technology (CN)
Affordable and clean energy
Openalex Percentile: Top 0%
Spectroscopy and Laser Applications
65.05
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Stepped-Type Photoacoustic Resonator for Simultaneous Dual-Gas Detection — Bingyu Mo, Hongchao Qi, et al. · Analytical Chemistry (2026) | TGRS Research Map | TGRS