Convective and inertial Marangoni surfing

We study the surfing motion of an active particle along a planar interface, separating a semi-infinite layer of gas from a deep layer of liquid. The interface-trapped particle self-propels, thanks to an uneven distribution of surface tension in its immediate vicinity, which itself results from a non-uniform release of an active agent from the particle’s surface. We use the reciprocal theorem in conjunction with singular perturbation expansions to calculate the leading-order contributions to the propulsion speed of the surfer due to the advective transport of mass and momentum when the Péclet and Reynolds numbers (denoted by $\textit{Pe}$ and $\textit{Re}$ , respectively) are small but finite. Assuming that the surface tension varies linearly with the concentration of the agent with a slope of negative $\alpha$ , we show, perhaps unexpectedly, that the normalised speed for a purely translating (but otherwise arbitrarily shaped) particle, independent of the agent discharge mechanism, can be expressed as $\mathscr{U} = 1 + \mathscr{A} ( 2 \textit{Pe} \ln \textit{Pe} + \textit{Re} \ln \textit{Re} ) + \mathscr{O}(\textit{Pe}) + \mathscr{O}(\textit{Re})$ , where the prefactor $\mathscr{A}$ is positive for negative $\alpha$ and vice versa . For reference, the self-propulsion speed of autophoretic Janus spheres varies with $\textit{Pe}$ as $\mathscr{U} = 1 + \mathscr{B} \, \textit{Pe} + {\cdots}$ , where $\mathscr{B}$ is positive when the mobility coefficient of the particle is negative and vice versa . Also, the speed of spherical squirmers changes with $\textit{Re}$ as $\mathscr{U} = 1 + \mathscr{C} \, \textit{Re} + \mathscr{O}(\textit{Re})^2$ , with $\mathscr{C}$ being positive for pushers and negative for pullers. Our asymptotic formula reveals that the speed of a Marangoni surfer is a non-monotonic function of the Péclet and Reynolds numbers, hinting at the existence of optimal values for both $\textit{Pe}$ and $\textit{Re}$ . The information contained within the multiplier $\mathscr{A}$ also offers guidance for customising the shape of the surfer, as well as the release rate and configuration of the agent, to enhance the self-surfing performance. Our general theoretical analysis is complemented by detailed numerical simulations for a representative spherical surfer. These simulations confirm our theoretical predictions and shed light on the effects of intermediate and large values of $\textit{Pe}$ and $\textit{Re}$ on the performance of Marangoni surfers.

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Publication Details

Journal
Journal of Fluid Mechanics
Published
2026-01-02
DOI
https://doi.org/10.1017/jfm.2025.11027
Primary Topic
Micro and Nano Robotics
Type
article
Field-Weighted Citation Impact
0.00

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article

Convective and inertial Marangoni surfing

Hassan Masoud, Esmaeil Dehdashti, Jonathan P. Rothstein, Saeed Jafari Kang
Journal of Fluid Mechanics
Micro and Nano Robotics
article

Convective and inertial Marangoni surfing

Hassan Masoud, Esmaeil Dehdashti, Jonathan P. Rothstein, Saeed Jafari Kang
article en

Abstract

We study the surfing motion of an active particle along a planar interface, separating a semi-infinite layer of gas from a deep layer of liquid. The interface-trapped particle self-propels, thanks to an uneven distribution of surface tension in its immediate vicinity, which itself results from a non-uniform release of an active agent from the particle’s surface. We use the reciprocal theorem in conjunction with singular perturbation expansions to calculate the leading-order contributions to the propulsion speed of the surfer due to the advective transport of mass and momentum when the Péclet and Reynolds numbers (denoted by $\textit{Pe}$ and $\textit{Re}$ , respectively) are small but finite. Assuming that the surface tension varies linearly with the concentration of the agent with a slope of negative $\alpha$ , we show, perhaps unexpectedly, that the normalised speed for a purely translating (but otherwise arbitrarily shaped) particle, independent of the agent discharge mechanism, can be expressed as $\mathscr{U} = 1 + \mathscr{A} ( 2 \textit{Pe} \ln \textit{Pe} + \textit{Re} \ln \textit{Re} ) + \mathscr{O}(\textit{Pe}) + \mathscr{O}(\textit{Re})$ , where the prefactor $\mathscr{A}$ is positive for negative $\alpha$ and vice versa . For reference, the self-propulsion speed of autophoretic Janus spheres varies with $\textit{Pe}$ as $\mathscr{U} = 1 + \mathscr{B} \, \textit{Pe} + {\cdots}$ , where $\mathscr{B}$ is positive when the mobility coefficient of the particle is negative and vice versa . Also, the speed of spherical squirmers changes with $\textit{Re}$ as $\mathscr{U} = 1 + \mathscr{C} \, \textit{Re} + \mathscr{O}(\textit{Re})^2$ , with $\mathscr{C}$ being positive for pushers and negative for pullers. Our asymptotic formula reveals that the speed of a Marangoni surfer is a non-monotonic function of the Péclet and Reynolds numbers, hinting at the existence of optimal values for both $\textit{Pe}$ and $\textit{Re}$ . The information contained within the multiplier $\mathscr{A}$ also offers guidance for customising the shape of the surfer, as well as the release rate and configuration of the agent, to enhance the self-surfing performance. Our general theoretical analysis is complemented by detailed numerical simulations for a representative spherical surfer. These simulations confirm our theoretical predictions and shed light on the effects of intermediate and large values of $\textit{Pe}$ and $\textit{Re}$ on the performance of Marangoni surfers.

Journal of Fluid MechanicsVol. 1026
Michigan Technological University (US), Clemson University (US)
National Science Foundation, Division of Chemical, Bioengineering, Environmental, and Transport Systems
Life below water
Openalex Percentile: Top 96%
Micro and Nano Robotics
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