Chirality-Induced Orbital-Angular-Momentum Selectivity in Electron Transmission and Scattering

Chirality-induced orbital-angular-momentum selectivity (CIOAMS) in electron transmission and scattering processes is investigated. Polarization of the OAM of an electron traversing chiral media is first studied via electronic wavepacket propagation using the time-dependent Schrödinger equation. Next, spatial resolution of wavepackets carrying opposite OAM, following scattering from a corrugated surface is demonstrated. This suggests that OAM may play a significant role in the mechanisms underlying chirality-induced spin selectivity, measured for electrons crossing chiral media in setups involving Mott polarimetry. Our results highlight the potential to exploit CIOAMS in innovative emerging quantum technologies.

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Publication Details

Journal
Journal of Chemical Theory and Computation
Published
2025-12-31
DOI
https://doi.org/10.1021/acs.jctc.5c01410
Primary Topic
Orbital Angular Momentum in Optics
Type
article
Field-Weighted Citation Impact
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article

Chirality-Induced Orbital-Angular-Momentum Selectivity in Electron Transmission and Scattering

Abraham Nitzan, Yun Chen, Joel I. Gersten, Oded Hod
Journal of Chemical Theory and Computation
Orbital Angular Momentum in Optics
article

Chirality-Induced Orbital-Angular-Momentum Selectivity in Electron Transmission and Scattering

Abraham Nitzan, Yun Chen, Joel I. Gersten, Oded Hod
article en

Abstract

Chirality-induced orbital-angular-momentum selectivity (CIOAMS) in electron transmission and scattering processes is investigated. Polarization of the OAM of an electron traversing chiral media is first studied via electronic wavepacket propagation using the time-dependent Schrödinger equation. Next, spatial resolution of wavepackets carrying opposite OAM, following scattering from a corrugated surface is demonstrated. This suggests that OAM may play a significant role in the mechanisms underlying chirality-induced spin selectivity, measured for electrons crossing chiral media in setups involving Mott polarimetry. Our results highlight the potential to exploit CIOAMS in innovative emerging quantum technologies.

Journal of Chemical Theory and ComputationVol. 22(1)
City College of New York (US), Tel Aviv University (IL), Exact Sciences (United States) (US), University of Pennsylvania (US)
Industry, innovation and infrastructure
Openalex Percentile: Top 30%
Orbital Angular Momentum in Optics
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