Transferable Plasmonic Arrays Enabling Strong Coupling with Layered Perovskites in an Active Diode Architecture

Plasmonic cavities provide a powerful platform for nanoscale light confinement far beyond the diffraction limit, enabling exceptionally strong light-matter interactions. Recent advances in plasmonic architectures and active materials enable stable, scalable routes toward fully integrated on-chip photonics. In this work, we demonstrate the strong coupling of 2D layered perovskites with a transferable plasmonic cavity directly fabricated on top of hexagonal boron nitride (hBN). Under optical excitation, we observe clear interaction between the exciton and cavity modes leading to strong and even ultrastrong coupling, with coupling factors <i>g</i> up to 10% of the resonance energy. Combined with the polariton mode hybridization and a waveguiding effect, this results in pronounced line width narrowing of the polariton modes well below both the bare cavity and exciton line widths. Electrical excitation of the hybrid modes is achieved via electron tunneling and simultaneous energy transfer, making this design an attractive configuration for on-chip integration.

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Publication Details

Journal
Nano Letters
Published
2025-12-31
DOI
https://doi.org/10.1021/acs.nanolett.5c04569
Primary Topic
Strong Light-Matter Interactions
Type
article
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article

Transferable Plasmonic Arrays Enabling Strong Coupling with Layered Perovskites in an Active Diode Architecture

L. Novotny, David J. Norris, Gabriel Nagamine, Kenji Watanabe et al.
Nano Letters
Strong Light-Matter Interactions
article

Transferable Plasmonic Arrays Enabling Strong Coupling with Layered Perovskites in an Active Diode Architecture

L. Novotny, David J. Norris, Gabriel Nagamine, Kenji Watanabe, Oleh R. Hordiichuk, T. Taniguchi, Antti Moilanen, Gabriele Rainò, Jonas D. Ziegler, Fabien Dorey, Maksym V. Kovalenko
article en

Abstract

Plasmonic cavities provide a powerful platform for nanoscale light confinement far beyond the diffraction limit, enabling exceptionally strong light-matter interactions. Recent advances in plasmonic architectures and active materials enable stable, scalable routes toward fully integrated on-chip photonics. In this work, we demonstrate the strong coupling of 2D layered perovskites with a transferable plasmonic cavity directly fabricated on top of hexagonal boron nitride (hBN). Under optical excitation, we observe clear interaction between the exciton and cavity modes leading to strong and even ultrastrong coupling, with coupling factors <i>g</i> up to 10% of the resonance energy. Combined with the polariton mode hybridization and a waveguiding effect, this results in pronounced line width narrowing of the polariton modes well below both the bare cavity and exciton line widths. Electrical excitation of the hybrid modes is achieved via electron tunneling and simultaneous energy transfer, making this design an attractive configuration for on-chip integration.

Nano LettersVol. 26(5)
University of Eastern Finland (FI), National Institute for Materials Science (JP), ETH Zurich (CH), Photonics (United States) (US), Finland University (FI), Institute of Inorganic Chemistry of the Slovak Academy of Sciences (SK), Department of Forestry (MW), Heinz Optical Engineering (United States) (US), Swiss Federal Laboratories for Materials Science and Technology (CH)
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Openalex Percentile: Top 30%
Strong Light-Matter Interactions
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