Nonreciprocal plasmons in one-dimensional carbon nanostructures

The directional control of light in miniaturized plasmonic waveguides holds appealing possibilities for emerging nanophotonic technologies, but is hindered by the intrinsic reciprocal optical response of conventional plasmonic materials. While the ability of graphene to sustain large electrical currents shows promise for nonreciprocal plasmonics, studies have been limited to extended samples characterized by linear electrical dispersion. Here, we theoretically explore quantum finite-size and nonlocal effects in the nonreciprocal response of mesoscale plasmonic waveguides comprised of drift-biased graphene nanoribbons (GNRs) and carbon nanotubes (CNTs). Using atomistic simulation methods based on tight-binding electronic states and self-consistent quantum mean-field optical response, we reveal that a moderate electrical bias can appreciably break reciprocity for propagation of guided plasmon modes in GNRs and CNTs exhibiting electronic band gaps. The excitation by a nearby point dipole emitter and subsequent propagation of guided plasmon modes can thus be actively controlled by the applied current, which can further be leveraged to mediate nonlocal interactions of multiple emitters. Our results establish graphene nanostructures as a promising atomically thin platform for nonreciprocal nanophotonics.

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Publication Details

Journal
Nature Communications
Published
2025-12-30
DOI
https://doi.org/10.1038/s41467-025-67872-5
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
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article

Nonreciprocal plasmons in one-dimensional carbon nanostructures

Joel D. Cox, Álvaro Rodríguez Echarri, F. Javier García de Abajo
Nature Communications
Plasmonic and Surface Plasmon Research
article

Nonreciprocal plasmons in one-dimensional carbon nanostructures

Joel D. Cox, Álvaro Rodríguez Echarri, F. Javier García de Abajo
article en

Abstract

The directional control of light in miniaturized plasmonic waveguides holds appealing possibilities for emerging nanophotonic technologies, but is hindered by the intrinsic reciprocal optical response of conventional plasmonic materials. While the ability of graphene to sustain large electrical currents shows promise for nonreciprocal plasmonics, studies have been limited to extended samples characterized by linear electrical dispersion. Here, we theoretically explore quantum finite-size and nonlocal effects in the nonreciprocal response of mesoscale plasmonic waveguides comprised of drift-biased graphene nanoribbons (GNRs) and carbon nanotubes (CNTs). Using atomistic simulation methods based on tight-binding electronic states and self-consistent quantum mean-field optical response, we reveal that a moderate electrical bias can appreciably break reciprocity for propagation of guided plasmon modes in GNRs and CNTs exhibiting electronic band gaps. The excitation by a nearby point dipole emitter and subsequent propagation of guided plasmon modes can thus be actively controlled by the applied current, which can further be leveraged to mediate nonlocal interactions of multiple emitters. Our results establish graphene nanostructures as a promising atomically thin platform for nonreciprocal nanophotonics.

Nature CommunicationsVol. 17(1)
Institució Catalana de Recerca i Estudis Avançats (ES), University of Southern Denmark (DK), Institute of Photonic Sciences (ES), Institute for Atomic and Molecular Physics (NL)
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Plasmonic and Surface Plasmon Research
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Nonreciprocal plasmons in one-dimensional carbon nanostructures — Joel D. Cox, Álvaro Rodríguez Echarri, et al. · Nature Communications (2025) | TGRS Research Map | TGRS