Unlocking High Coercivity at Room Temperature in Phase Modified MoS <sub>2</sub>

2D materials showing room-temperature magnetism and high coercivity are highly attractive for combining magnetism with semiconducting functionality in spintronic devices. In this work, the magnetic properties of the 1T phase of MoS<sub>2</sub> have been studied at room temperature. We observe ferromagnetism with a coercivity of ∼0.3 T and a maximum saturation magnetization of 0.26 emu g<sup>-1</sup> at room temperature. This is the highest among coercivities reported so far in 2D magnets at room temperature. MoS<sub>2</sub> nanosheets are prepared using a single-step hydrothermal synthesis with a relative 1T-phase reaching up to 77%. Structural analysis reveals lattice expansion, reflected by an increased interplanar spacing, which correlates directly with both the relative 1T phase fraction and enhanced coercivity. Our findings demonstrate a direct structural route to engineer coercivity through phase and strain control in MoS<sub>2</sub>, offering a scalable platform for phase-engineered magnetism in layered materials.

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Journal
Small
Published
2025-12-26
DOI
https://doi.org/10.1002/smll.202509637
Primary Topic
2D Materials and Applications
Type
article
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Unlocking High Coercivity at Room Temperature in Phase Modified MoS 2

Kushal Mazumder, Pramoda Kumar Nayak, Zainab Chowdhry, Ajit K. Jena et al.
Small
2D Materials and Applications
article

Unlocking High Coercivity at Room Temperature in Phase Modified MoS 2

Kushal Mazumder, Pramoda Kumar Nayak, Zainab Chowdhry, Ajit K. Jena, Vidya Praveen Bhallamudi, Praveen Hegde
article en

Abstract

2D materials showing room-temperature magnetism and high coercivity are highly attractive for combining magnetism with semiconducting functionality in spintronic devices. In this work, the magnetic properties of the 1T phase of MoS<sub>2</sub> have been studied at room temperature. We observe ferromagnetism with a coercivity of ∼0.3 T and a maximum saturation magnetization of 0.26 emu g<sup>-1</sup> at room temperature. This is the highest among coercivities reported so far in 2D magnets at room temperature. MoS<sub>2</sub> nanosheets are prepared using a single-step hydrothermal synthesis with a relative 1T-phase reaching up to 77%. Structural analysis reveals lattice expansion, reflected by an increased interplanar spacing, which correlates directly with both the relative 1T phase fraction and enhanced coercivity. Our findings demonstrate a direct structural route to engineer coercivity through phase and strain control in MoS<sub>2</sub>, offering a scalable platform for phase-engineered magnetism in layered materials.

SmallVol. 22(9)
Jain University (IN), Indian Institute of Technology Madras (IN), Noida International University (IN), Indo Korea Science and Technology (IN)
Openalex Percentile: Top 48%
2D Materials and Applications
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