Single-Particle Photothermal Microscopy Using On-Chip Silicon Nitride Microring Resonators

Optical microresonators confine light in time and space, enabling high sensitivity for the detection of small thermal perturbations. We utilized these properties and investigated on-chip integrated silicon nitride microring resonators (MRRs) for single-particle photothermal microscopy. We calibrate the technique using individual nonphotoluminescent carbon nanotubes and determine values for absorption cross-section per atom that agree with literature values. Finite-element simulations are performed to track all relevant thermal gradients. The combination of experiment and simulation allows for discussion of the benefits and drawbacks of the planar MRR geometry for single-particle microscopy.

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Publication Details

Journal
The Journal of Physical Chemistry A
Published
2025-12-24
DOI
https://doi.org/10.1021/acs.jpca.5c06077
Primary Topic
Mechanical and Optical Resonators
Type
article
Field-Weighted Citation Impact
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article

Single-Particle Photothermal Microscopy Using On-Chip Silicon Nitride Microring Resonators

Randall H. Goldsmith, Arka Majumdar, Sam Evans, Arnab Manna et al.
The Journal of Physical Chemistry A
Mechanical and Optical Resonators
article

Single-Particle Photothermal Microscopy Using On-Chip Silicon Nitride Microring Resonators

Randall H. Goldsmith, Arka Majumdar, Sam Evans, Arnab Manna, Cecilia H. Vollbrecht, Hannah Rarick, Yulia Podorova
article en

Abstract

Optical microresonators confine light in time and space, enabling high sensitivity for the detection of small thermal perturbations. We utilized these properties and investigated on-chip integrated silicon nitride microring resonators (MRRs) for single-particle photothermal microscopy. We calibrate the technique using individual nonphotoluminescent carbon nanotubes and determine values for absorption cross-section per atom that agree with literature values. Finite-element simulations are performed to track all relevant thermal gradients. The combination of experiment and simulation allows for discussion of the benefits and drawbacks of the planar MRR geometry for single-particle microscopy.

The Journal of Physical Chemistry AVol. 130(1)
University of Wisconsin–Madison (US), University of Washington (US)
Openalex Percentile: Top 32%
Mechanical and Optical Resonators
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