One-Dimensional Simulation of PM Deposition and Regeneration in Particulate Filters: Optimal Conditions for PM Oxidation in GPF Considering Oxygen Concentration and Temperature

This study presents a one-dimensional numerical simulation of particulate matter (PM) oxidation and regeneration behavior in gasoline particulate filters (GPFs) under Worldwide Harmonized Light Vehicles Test Cycle (WLTC) conditions. The model incorporates both catalyst activity—represented by activation energy (E) and pre-exponential factor (A)—and exhaust control strategies involving forced fuel cut (FC). PM deposition and oxidation were simulated based on solid-state and gas-phase reactions, with the effects of oxygen concentration and temperature analyzed in detail. The results show that under high catalyst activity (E = 100 kJ mol−1, A = 6.2 × 107), PM oxidation proceeds efficiently even during medium-speed phases, achieving a 98.8% oxidation rate after one WLTC. Conversely, conventional catalysts (E = 120 kJ mol−1, A = 6.2 × 106) exhibited limited regeneration, leaving 0.11 g of residual PM. Introducing forced FC effectively enhanced oxidation by increasing oxygen concentration to 20% and sustaining heat release. A single continuous 100 s FC yielded the highest oxidation (96% reduction), while split FCs reduced peak PM accumulation. These findings demonstrate that optimizing the balance between catalyst activity and FC control can significantly improve GPF regeneration performance, providing a practical strategy for PM reduction in GDI vehicles under real driving conditions.

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Publication Details

Journal
Applied Sciences
Published
2025-12-23
DOI
https://doi.org/10.3390/app16010150
Primary Topic
Catalytic Processes in Materials Science
Type
article
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article

One-Dimensional Simulation of PM Deposition and Regeneration in Particulate Filters: Optimal Conditions for PM Oxidation in GPF Considering Oxygen Concentration and Temperature

Masanao Ozawa, Maki Nakamura, Koji Yokota
Applied Sciences
Catalytic Processes in Materials Science
article

One-Dimensional Simulation of PM Deposition and Regeneration in Particulate Filters: Optimal Conditions for PM Oxidation in GPF Considering Oxygen Concentration and Temperature

Masanao Ozawa, Maki Nakamura, Koji Yokota
article en

Abstract

This study presents a one-dimensional numerical simulation of particulate matter (PM) oxidation and regeneration behavior in gasoline particulate filters (GPFs) under Worldwide Harmonized Light Vehicles Test Cycle (WLTC) conditions. The model incorporates both catalyst activity—represented by activation energy (E) and pre-exponential factor (A)—and exhaust control strategies involving forced fuel cut (FC). PM deposition and oxidation were simulated based on solid-state and gas-phase reactions, with the effects of oxygen concentration and temperature analyzed in detail. The results show that under high catalyst activity (E = 100 kJ mol−1, A = 6.2 × 107), PM oxidation proceeds efficiently even during medium-speed phases, achieving a 98.8% oxidation rate after one WLTC. Conversely, conventional catalysts (E = 120 kJ mol−1, A = 6.2 × 106) exhibited limited regeneration, leaving 0.11 g of residual PM. Introducing forced FC effectively enhanced oxidation by increasing oxygen concentration to 20% and sustaining heat release. A single continuous 100 s FC yielded the highest oxidation (96% reduction), while split FCs reduced peak PM accumulation. These findings demonstrate that optimizing the balance between catalyst activity and FC control can significantly improve GPF regeneration performance, providing a practical strategy for PM reduction in GDI vehicles under real driving conditions.

Applied SciencesVol. 16(1)
Nagoya University (JP)
Affordable and clean energy
Openalex Percentile: Top 49%
Catalytic Processes in Materials Science
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