Low-Field Optical Polarization in Type-II Quantum Dots via Nuclear-Driven Dark State Mixing

Semiconductor quantum dots (QDs) offer a rich landscape for spin control and quantum light emission. While most studies have focused on type-I band alignment, the potential of type-II systems remains underexplored. Here, we report low-field optical polarization in type-II In(Ga)As/GaAsSb QDs, enabled by hyperfine-induced mixing between bright and dark excitons via level anticrossing under magnetic fields as low as 0.17 T. The weak-field regime arises from the suppressed wave function overlap, yielding a reduced electron-hole exchange interaction. A theoretical model based on the spin Hamiltonian and the spin-split state populations accurately captures the observed mirror-symmetric luminescence helicity, reproducing the experimental polarization response. Additionally, polarization recovery measurements confirm the role of nuclear spin interactions in mediating the in-plane electron spin precession. Our work demonstrates an alternative route for light polarization control using weak magnetic fields and nonresonant linear excitation, establishing type-II QDs as promising platforms for compact sources of circularly polarized light.

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Publication Details

Journal
Nano Letters
Published
2025-12-22
DOI
https://doi.org/10.1021/acs.nanolett.5c05163
Primary Topic
Quantum and electron transport phenomena
Type
article
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article

Low-Field Optical Polarization in Type-II Quantum Dots via Nuclear-Driven Dark State Mixing

Victor Lopez‐Richard, Marcio Daldin Teodoro, Morgan E. Ware, Gabriel Jacobsen et al.
Nano Letters
Quantum and electron transport phenomena
article

Low-Field Optical Polarization in Type-II Quantum Dots via Nuclear-Driven Dark State Mixing

Victor Lopez‐Richard, Marcio Daldin Teodoro, Morgan E. Ware, Gabriel Jacobsen, Vinicius Antonio de Oliveira, G. E. Marques, Baolai Liang, Yuriy I. Mazur, Gregory J. Salamo
article en

Abstract

Semiconductor quantum dots (QDs) offer a rich landscape for spin control and quantum light emission. While most studies have focused on type-I band alignment, the potential of type-II systems remains underexplored. Here, we report low-field optical polarization in type-II In(Ga)As/GaAsSb QDs, enabled by hyperfine-induced mixing between bright and dark excitons via level anticrossing under magnetic fields as low as 0.17 T. The weak-field regime arises from the suppressed wave function overlap, yielding a reduced electron-hole exchange interaction. A theoretical model based on the spin Hamiltonian and the spin-split state populations accurately captures the observed mirror-symmetric luminescence helicity, reproducing the experimental polarization response. Additionally, polarization recovery measurements confirm the role of nuclear spin interactions in mediating the in-plane electron spin precession. Our work demonstrates an alternative route for light polarization control using weak magnetic fields and nonresonant linear excitation, establishing type-II QDs as promising platforms for compact sources of circularly polarized light.

Nano LettersVol. 26(1)
California NanoSystems Institute (US), University of California, Los Angeles (US), Universidade Federal de São Carlos (BR), Center for NanoScience (DE), University of Arkansas at Fayetteville (US)
Openalex Percentile: Top 33%
Quantum and electron transport phenomena
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