Light wave induced nanosecond-long persistent state in the Dirac semimetal <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Cd</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi>As</mml:mi> <mml:mn>2</mm

Unraveling light induced ultrafast dynamics in three-dimensional Dirac materials is crucial for deepening our fundamental understanding and for advancing potential optoelectronic applications. While time-resolved pump-probe spectroscopy has predominantly revealed carrier dynamics governed by Dirac fermion cooling and population inversion, the full picture of relaxation pathways remains incomplete. In this Letter, we identify a relaxation channel in these materials. Using strong terahertz (THz) field excitation combined with a near-infrared (NIR) probe, we detect a long-lived carrier population persisting on the nanosecond timescale. This extended lifetime suggests that carriers become trapped in defect states, leading to sub-band-gap absorption in the NIR and pointing to the significant role of defect-assisted relaxation in the carrier dynamics of Dirac semimetals.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-12-22
DOI
https://doi.org/10.1103/yj4s-7ks7
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
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article

Light wave induced nanosecond-long persistent state in the Dirac semimetal <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Cd</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi>As</mml:mi> <mml:mn>2</mm

Anonymous
Physical review. B./Physical review. B
Topological Materials and Phenomena
article

Light wave induced nanosecond-long persistent state in the Dirac semimetal <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Cd</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi>As</mml:mi> <mml:mn>2</mm

Anonymous
article en

Abstract

Unraveling light induced ultrafast dynamics in three-dimensional Dirac materials is crucial for deepening our fundamental understanding and for advancing potential optoelectronic applications. While time-resolved pump-probe spectroscopy has predominantly revealed carrier dynamics governed by Dirac fermion cooling and population inversion, the full picture of relaxation pathways remains incomplete. In this Letter, we identify a relaxation channel in these materials. Using strong terahertz (THz) field excitation combined with a near-infrared (NIR) probe, we detect a long-lived carrier population persisting on the nanosecond timescale. This extended lifetime suggests that carriers become trapped in defect states, leading to sub-band-gap absorption in the NIR and pointing to the significant role of defect-assisted relaxation in the carrier dynamics of Dirac semimetals.

Physical review. B./Physical review. BVol. 113(4)
TU Dortmund University (DE), Fudan University (CN), Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE), Korea Institute of Science and Technology (KR)
Openalex Percentile: Top 33%
Topological Materials and Phenomena
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