Ultrafast Raman probe of the photoinduced superconducting to normal state transition in the cuprate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Bi</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>
We report an ultrafast Time-Resolved Raman scattering study of the out-of-equilibrium photoinduced dynamics across the superconducting to normal state phase transition of the cuprate Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. Using the polarization-resolved momentum space selectivity of Raman scattering, we track the superconducting condensate destruction and recovery dynamics with sub-picoseconds time resolution in the anti-nodal region of the Fermi surface where the superconducting gap is maximum. Leveraging ultrafast Raman thermometry, we find a significant dichotomy between the superconducting condensate and the quasiparticle temperature dynamics near the anti-nodes, which cannot be framed in terms of a single effective electron temperature. The present work demonstrates the ability of Time-Resolved Raman scattering to selectively probe out-of-equilibrium pathways of different electronic sub-degrees of freedom during a photoinduced phase transition.
Institutions
- Institut Universitaire de France (FR)
- Université Paris Cité (FR)
- Laboratoire Matériaux et Phénomènes Quantiques (FR)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-12-17
- DOI
- https://doi.org/10.1103/wkx7-lcqf
- Primary Topic
- Physics of Superconductivity and Magnetism
- Type
- article
- Field-Weighted Citation Impact
- 0.00