Intrinsic low-temperature magnetic properties on ultraclean UTe₂ with 𝑇𝑐=2.1 K revealed by ¹²⁵Te NMR

To investigate the intrinsic magnetic properties of UTe₂, we performed ¹²⁵Te-NMR measurements on the ultraclean single-crystalline UTe₂ with superconducting transition temperature 𝑇𝑐=2.1 K and compared the results with those of the 𝑇𝑐=1.6 K sample. The broadening of the linewidth of the NMR spectrum in the 𝑎-axis magnetic field and the low-temperature magnetic fluctuations observed in the 1.6 K sample are suppressed in the ultraclean sample, indicating that such magnetic properties originate from a tiny amount of U deficiency. The present results suggest that the magnetic properties in UTe₂ are sensitive to the U deficiency. We also observed a peculiar angular dependence of the NMR quantities due to large magnetic anisotropy with the 𝑎 axis as the magnetic easy axis.

Publication Details

Journal
Kyoto University Research Information Repository (Kyoto University)
Published
2025-03-10
Primary Topic
Rare-earth and actinide compounds
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article
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article

Intrinsic low-temperature magnetic properties on ultraclean UTe₂ with 𝑇𝑐=2.1 K revealed by ¹²⁵Te NMR

Kyoto University Research Information Repository (Kyoto University)
Rare-earth and actinide compounds
article

Intrinsic low-temperature magnetic properties on ultraclean UTe₂ with 𝑇𝑐=2.1 K revealed by ¹²⁵Te NMR

article en

Abstract

To investigate the intrinsic magnetic properties of UTe₂, we performed ¹²⁵Te-NMR measurements on the ultraclean single-crystalline UTe₂ with superconducting transition temperature 𝑇𝑐=2.1 K and compared the results with those of the 𝑇𝑐=1.6 K sample. The broadening of the linewidth of the NMR spectrum in the 𝑎-axis magnetic field and the low-temperature magnetic fluctuations observed in the 1.6 K sample are suppressed in the ultraclean sample, indicating that such magnetic properties originate from a tiny amount of U deficiency. The present results suggest that the magnetic properties in UTe₂ are sensitive to the U deficiency. We also observed a peculiar angular dependence of the NMR quantities due to large magnetic anisotropy with the 𝑎 axis as the magnetic easy axis.

Kyoto University Research Information Repository (Kyoto University)
Openalex Percentile: Top 32%
Rare-earth and actinide compounds
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Intrinsic low-temperature magnetic properties on ultraclean UTe₂ with 𝑇𝑐=2.1 K revealed by ¹²⁵Te NMR · Kyoto University Research Information Repository (Kyoto University) (2025) | TGRS Research Map | TGRS