A signal-processing framework for preemptive detection of soft shorts in lithium-metal batteries

<h2>Summary</h2> Lithium-ion batteries are central to sustainable energy systems, yet internal short circuits (ISCs) can trigger catastrophic failures, such as fires and explosions. Current detection methods are based on costly tests, large datasets, or computationally heavy models, which limit their scalability and practical application. Here, we report a physics-based framework for the early detection of soft ISCs by representing the battery as an equivalent resistance-capacitance (RC) circuit with time-varying resistances. Using signal processing, we track periodic resistance fluctuations in charging data to identify the onset of ISCs without any abuse conditions. Fast Fourier transform (FFT) highlights distinct frequency-domain signatures, while Welch's algorithm extracts characteristic power spectral density patterns that serve as detection criteria. Together, these methods provide robust, real-time monitoring of ISC formation. Our results establish a new diagnostic standard that links microscopic ISC dynamics with macroscopic signals, significantly improving battery safety for electric vehicles, consumer electronics, and grid-scale energy storage.

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Publication Details

Journal
Cell Reports Physical Science
Published
2025-11-24
DOI
https://doi.org/10.1016/j.xcrp.2025.102973
Primary Topic
Advanced Battery Technologies Research
Type
article
Field-Weighted Citation Impact
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article

A signal-processing framework for preemptive detection of soft shorts in lithium-metal batteries

Cell Reports Physical Science
Advanced Battery Technologies Research
article

A signal-processing framework for preemptive detection of soft shorts in lithium-metal batteries

article en

Abstract

<h2>Summary</h2> Lithium-ion batteries are central to sustainable energy systems, yet internal short circuits (ISCs) can trigger catastrophic failures, such as fires and explosions. Current detection methods are based on costly tests, large datasets, or computationally heavy models, which limit their scalability and practical application. Here, we report a physics-based framework for the early detection of soft ISCs by representing the battery as an equivalent resistance-capacitance (RC) circuit with time-varying resistances. Using signal processing, we track periodic resistance fluctuations in charging data to identify the onset of ISCs without any abuse conditions. Fast Fourier transform (FFT) highlights distinct frequency-domain signatures, while Welch's algorithm extracts characteristic power spectral density patterns that serve as detection criteria. Together, these methods provide robust, real-time monitoring of ISC formation. Our results establish a new diagnostic standard that links microscopic ISC dynamics with macroscopic signals, significantly improving battery safety for electric vehicles, consumer electronics, and grid-scale energy storage.

Cell Reports Physical ScienceVol. 6(12)
Ming Chi University of Technology (TW), National Taiwan University of Science and Technology (TW), National Synchrotron Radiation Research Center (TW)
Openalex Percentile: Top 49%
Advanced Battery Technologies Research
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