Local Symmetry Broken, Global Spins Aligned: Co-Emergence of Local Distortions and Antiferromagnetism in the Kagome Magnet (Fe0.55Co0.45)Sn

Kagome-lattice materials, such as CoSn and FeSn, have attracted significant interest as hosts of electronic flat bands and topological properties, yet their behaviors are primarily understood through average crystal structures. Here, we report the co-emergence of antiferromagnetic (AFM) order and local symmetry breaking in nominal (Fe0.55Co0.45)Sn. Using a combination of neutron powder diffraction, synchrotron x-ray total scattering, and reverse Monte Carlo modeling, we uncover simultaneous magnetic ordering and local orthorhombic distortion below TN = 140 K. In this presentation, I will share comprehensive neutron and synchrotron x-ray scattering results, along with detailed analysis of short-range correlations. Our findings demonstrate that local symmetry breaking is unexpectedly coupled to global magnetic ordering, offering new insights into the interplay between structural and magnetic degrees of freedom in kagome magnets.

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Publication Details

Journal
Structural Dynamics
Published
2025-09-01
DOI
https://doi.org/10.1063/4.0000797
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
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article

Local Symmetry Broken, Global Spins Aligned: Co-Emergence of Local Distortions and Antiferromagnetism in the Kagome Magnet (Fe0.55Co0.45)Sn

Structural Dynamics
Topological Materials and Phenomena
article

Local Symmetry Broken, Global Spins Aligned: Co-Emergence of Local Distortions and Antiferromagnetism in the Kagome Magnet (Fe0.55Co0.45)Sn

article en

Abstract

Kagome-lattice materials, such as CoSn and FeSn, have attracted significant interest as hosts of electronic flat bands and topological properties, yet their behaviors are primarily understood through average crystal structures. Here, we report the co-emergence of antiferromagnetic (AFM) order and local symmetry breaking in nominal (Fe0.55Co0.45)Sn. Using a combination of neutron powder diffraction, synchrotron x-ray total scattering, and reverse Monte Carlo modeling, we uncover simultaneous magnetic ordering and local orthorhombic distortion below TN = 140 K. In this presentation, I will share comprehensive neutron and synchrotron x-ray scattering results, along with detailed analysis of short-range correlations. Our findings demonstrate that local symmetry breaking is unexpectedly coupled to global magnetic ordering, offering new insights into the interplay between structural and magnetic degrees of freedom in kagome magnets.

Structural DynamicsVol. 12(5_Supplement)
Oak Ridge National Laboratory (US)
Peace, Justice and strong institutions
Openalex Percentile: Top 44%
Topological Materials and Phenomena
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Local Symmetry Broken, Global Spins Aligned: Co-Emergence of Local Distortions and Antiferromagnetism in the Kagome Magnet (Fe0.55Co0.45)Sn · Structural Dynamics (2025) | TGRS Research Map | TGRS