Atomically-defined on-surface synthesis of multilayer metal-organic frameworks

This experimental and computational dataset contains the raw underlying data for the article "Atomically-defined on-surface synthesis of multilayer metal-organic frameworks" published in Communications Chemistry. The details of the sample preparation, data analysis and interpretation are given in the published article. The authors ackonwledge funding from the Czech Science Foundation (GAČR grant 24-10593L), from MEYS CR (CzechNanoLab project LM2023051, IMPROVE V, CZ.02.01.01/00/22_010/0002552 and e-INFRA CZ ID: 90140) and from the European Union's Horizon Widera 2022 program (grant agreement No. 101130765). The DFT computations were carried out at IT4I National Supercomputing Center.