Field-tuning of ultrafast magnetization fluctuations in Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$

The properties of spin fluctuations in antiferromagnets are largely unexplored, in particular at ultrafast timescales. Here, we employ femtosecond noise correlation spectroscopy (FemNoC) to experimentally study magnetization fluctuations in the canted antiferromagnet Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$ across its spin reorientation transition and under external magnetic fields. By comparing our measurements to atomistic spin noise and Monte Carlo simulations, we find that the amplitude of the spin noise is governed by the free energy, with stronger fluctuations in regions where the potential landscape softens. We furthermore demonstrate that external magnetic fields suppress spin fluctuations and enhance the quasi-ferromagnetic magnon frequency by effectively stiffening the potential. These results highlight an effective route for tuning ultrafast magnetization fluctuations via external parameters.

Publication Details

Journal
ArXiv.org
Published
2025-09-30
Primary Topic
Geology and Paleoclimatology Research
Type
article
Field-Weighted Citation Impact
0.00

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article

Field-tuning of ultrafast magnetization fluctuations in Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$

ArXiv.org
Geology and Paleoclimatology Research
article

Field-tuning of ultrafast magnetization fluctuations in Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$

article en

Abstract

The properties of spin fluctuations in antiferromagnets are largely unexplored, in particular at ultrafast timescales. Here, we employ femtosecond noise correlation spectroscopy (FemNoC) to experimentally study magnetization fluctuations in the canted antiferromagnet Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$ across its spin reorientation transition and under external magnetic fields. By comparing our measurements to atomistic spin noise and Monte Carlo simulations, we find that the amplitude of the spin noise is governed by the free energy, with stronger fluctuations in regions where the potential landscape softens. We furthermore demonstrate that external magnetic fields suppress spin fluctuations and enhance the quasi-ferromagnetic magnon frequency by effectively stiffening the potential. These results highlight an effective route for tuning ultrafast magnetization fluctuations via external parameters.

ArXiv.org
Deutsche Forschungsgemeinschaft, Universität Konstanz, Japan Society for the Promotion of Science
Affordable and clean energy
Openalex Percentile: Top 41%
Geology and Paleoclimatology Research
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