Splitting of electronic spectrum in paramagnetic phase of itinerant ferromagnets and altermagnets

We study self-energy effects induced by strong magnetic fluctuations in the paramagnetic phase of strongly-correlated itinerant magnets within the density functional theory combined with the dynamical mean field theory (DFT+DMFT approach) and its non-local extension. We show that both local and non-local magnetic correlations yield a splitting of the electronic spectrum in the paramagnetic phase, such that it closely resembles the DFT band structure in the ordered phase. We demonstrate these effects on $α$-iron, half-metal CrO$_2$, van der Waals material CrTe$_2$, and altermagnet CrSb. Although the obtained split bands do not possess a certain spin projection, their splitting suppresses spectral weight at the Fermi level. Even when originating from local magnetic correlations, the splitting is strongly momentum dependent as a consequence of the orbital selectivity of non-quasiparticle states. The relative importance of non-local vs. local correlations depends on the proximity to half filling of $d$ states: closer to half filling, the role of local correlations increases.

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ArXiv.org
Published
2025-09-27
Primary Topic
Cell Image Analysis Techniques
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article

Splitting of electronic spectrum in paramagnetic phase of itinerant ferromagnets and altermagnets

ArXiv.org
Cell Image Analysis Techniques
article

Splitting of electronic spectrum in paramagnetic phase of itinerant ferromagnets and altermagnets

article en

Abstract

We study self-energy effects induced by strong magnetic fluctuations in the paramagnetic phase of strongly-correlated itinerant magnets within the density functional theory combined with the dynamical mean field theory (DFT+DMFT approach) and its non-local extension. We show that both local and non-local magnetic correlations yield a splitting of the electronic spectrum in the paramagnetic phase, such that it closely resembles the DFT band structure in the ordered phase. We demonstrate these effects on $α$-iron, half-metal CrO$_2$, van der Waals material CrTe$_2$, and altermagnet CrSb. Although the obtained split bands do not possess a certain spin projection, their splitting suppresses spectral weight at the Fermi level. Even when originating from local magnetic correlations, the splitting is strongly momentum dependent as a consequence of the orbital selectivity of non-quasiparticle states. The relative importance of non-local vs. local correlations depends on the proximity to half filling of $d$ states: closer to half filling, the role of local correlations increases.

ArXiv.org
Moscow Institute of Physics and Technology (RU)
Affordable and clean energy
Openalex Percentile: Top 36%
Cell Image Analysis Techniques
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