Extended Data for In Situ Method for Quantifying Tritium Production from <sup>10</sup>B(n, t+2α) Using Boron Loaded Scintillator

Accurate neutron cross section data is important for nuclear science applications, including modeling, benchmarking, and reactor design. For the <sup>10</sup>B channel, the production of tritium through fast neutron reactions on <sup>10</sup>B is of interest for both nuclear data and fuel cycles applications. Current cross section data for the <sup>10</sup>B channel is sparse and inconsistent, making it difficult to evaluate this reaction with confidence. This work reviews the current state of both experimental and evaluated nuclear data for the reaction. We propose a simple in situ measurement methodology in which boron loaded liquid scintillator is irradiated with 14.1 MeV neutrons, and tritium is quantified directly by liquid scintillation counting in the same sealed vial. This eliminates the need for chemical separation and minimizes experimental complexity. Preliminary calculations indicate that, under realistic irradiation conditions, the setup can generate measurable tritium activity above established detection limits for low background liquid scintillation techniques. Simulations confirm that the thin target approximation is reasonable for a 5 wt% boron solution.

Publication Details

Journal
Figshare
Published
2025-09-24
DOI
https://doi.org/10.6084/m9.figshare.30204094
Primary Topic
Geochemistry and Geologic Mapping
Type
article
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article

Extended Data for In Situ Method for Quantifying Tritium Production from 10B(n, t+2α) Using Boron Loaded Scintillator

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Geochemistry and Geologic Mapping
article

Extended Data for In Situ Method for Quantifying Tritium Production from 10B(n, t+2α) Using Boron Loaded Scintillator

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Abstract

Accurate neutron cross section data is important for nuclear science applications, including modeling, benchmarking, and reactor design. For the <sup>10</sup>B channel, the production of tritium through fast neutron reactions on <sup>10</sup>B is of interest for both nuclear data and fuel cycles applications. Current cross section data for the <sup>10</sup>B channel is sparse and inconsistent, making it difficult to evaluate this reaction with confidence. This work reviews the current state of both experimental and evaluated nuclear data for the reaction. We propose a simple in situ measurement methodology in which boron loaded liquid scintillator is irradiated with 14.1 MeV neutrons, and tritium is quantified directly by liquid scintillation counting in the same sealed vial. This eliminates the need for chemical separation and minimizes experimental complexity. Preliminary calculations indicate that, under realistic irradiation conditions, the setup can generate measurable tritium activity above established detection limits for low background liquid scintillation techniques. Simulations confirm that the thin target approximation is reasonable for a 5 wt% boron solution.

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Geochemistry and Geologic Mapping
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Extended Data for In Situ Method for Quantifying Tritium Production from <sup>10</sup>B(n, t+2α) Using Boron Loaded Scintillator · Figshare (2025) | TGRS Research Map | TGRS