What causes the variation in superconducting properties of UTe$_{2}$?

Reaching a consensus on the superconducting order parameter of unconventional superconductors remains a central challenge in the field of magnetically-mediated superconductivity. Though UTe$_{2}$ is largely accepted as a rare example of an odd-parity superconductor, its precise order parameter remains highly debated, even at ambient conditions. A key underlying issue is the large sample-to-sample variation in superconducting properties at zero applied pressure and magnetic field. Here, we investigate the origin of the observed variation by means of single crystal x-ray diffraction (SC-XRD) and scanning transmission electron microscopy (STEM) measurements. Our results reveal highly ordered crystalline lattices, in agreement with the expected $Immm$ structure, and no signs of uranium vacancies. Tiny amounts of interstitial defects, however, are observed on the Te2 layers that host Te chains along the b axis. We argue that these defects give rise to slightly enhanced atomic displacement parameters observed in SC-XRD data and are enough to disrupt the unconventional superconducting state in UTe$_{2}$. Our findings highlight the need to focus future order parameter determination efforts on single crystals of UTe$_{2}$ with minimal amounts of structural disorder.

Publication Details

Journal
ArXiv.org
Published
2025-09-24
Primary Topic
Geochemistry and Geologic Mapping
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article
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article

What causes the variation in superconducting properties of UTe$_{2}$?

ArXiv.org
Geochemistry and Geologic Mapping
article

What causes the variation in superconducting properties of UTe$_{2}$?

article en

Abstract

Reaching a consensus on the superconducting order parameter of unconventional superconductors remains a central challenge in the field of magnetically-mediated superconductivity. Though UTe$_{2}$ is largely accepted as a rare example of an odd-parity superconductor, its precise order parameter remains highly debated, even at ambient conditions. A key underlying issue is the large sample-to-sample variation in superconducting properties at zero applied pressure and magnetic field. Here, we investigate the origin of the observed variation by means of single crystal x-ray diffraction (SC-XRD) and scanning transmission electron microscopy (STEM) measurements. Our results reveal highly ordered crystalline lattices, in agreement with the expected $Immm$ structure, and no signs of uranium vacancies. Tiny amounts of interstitial defects, however, are observed on the Te2 layers that host Te chains along the b axis. We argue that these defects give rise to slightly enhanced atomic displacement parameters observed in SC-XRD data and are enough to disrupt the unconventional superconducting state in UTe$_{2}$. Our findings highlight the need to focus future order parameter determination efforts on single crystals of UTe$_{2}$ with minimal amounts of structural disorder.

ArXiv.org
Openalex Percentile: Top 26%
Geochemistry and Geologic Mapping
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What causes the variation in superconducting properties of UTe$_{2}$? · ArXiv.org (2025) | TGRS Research Map | TGRS