X-ray magnetic circular dichroism originating from the $T_{z}$ term in collinear altermagnets under trigonal crystal field

We investigate the microscopic origin and spectral features of X-ray magnetic circular dichroism (XMCD) in collinear antiferromagnets with trigonal crystal fields, using $α$-MnTe as a prototypical example. Although such systems exhibit zero net magnetization, we demonstrate that XMCD can emerge from the anisotropic magnetic dipole operator $T_{z}$, arising from quadrupolar spin distributions. By constructing a complete multipole basis and analyzing the symmetry conditions under trigonal distortion, we identify specific spin and orbital configurations that enable a finite XMCD response. Further, we employ both one-electron and multi-electron models, including spin-orbit coupling and Coulomb interactions, to calculate the XMCD spectra for various $d^n$ configurations. Our findings provide theoretical benchmarks for XMCD in altermagnets and highlight the key role of orbital symmetry and magnetic anisotropy in realizing observable dichroic effects.

Publication Details

Journal
ArXiv.org
Published
2025-08-25
Primary Topic
Geochemistry and Geologic Mapping
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article
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article

X-ray magnetic circular dichroism originating from the $T_{z}$ term in collinear altermagnets under trigonal crystal field

ArXiv.org
Geochemistry and Geologic Mapping
article

X-ray magnetic circular dichroism originating from the $T_{z}$ term in collinear altermagnets under trigonal crystal field

article en

Abstract

We investigate the microscopic origin and spectral features of X-ray magnetic circular dichroism (XMCD) in collinear antiferromagnets with trigonal crystal fields, using $α$-MnTe as a prototypical example. Although such systems exhibit zero net magnetization, we demonstrate that XMCD can emerge from the anisotropic magnetic dipole operator $T_{z}$, arising from quadrupolar spin distributions. By constructing a complete multipole basis and analyzing the symmetry conditions under trigonal distortion, we identify specific spin and orbital configurations that enable a finite XMCD response. Further, we employ both one-electron and multi-electron models, including spin-orbit coupling and Coulomb interactions, to calculate the XMCD spectra for various $d^n$ configurations. Our findings provide theoretical benchmarks for XMCD in altermagnets and highlight the key role of orbital symmetry and magnetic anisotropy in realizing observable dichroic effects.

ArXiv.org
Openalex Percentile: Top 64%
Geochemistry and Geologic Mapping
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