X-ray-induced quenching of the $^{229}$Th clock isomer in CaF$_2$

Thorium-229 has the lowest nuclear-excited state (an isomer state) at approximately 8.356 eV, making it excitable with tabletop vacuum-ultraviolet lasers. Despite the recent success of laser excitation, the isomer quenching inside the solid-state environment remains unresolved. In this letter, we present experiments investigating X-ray-induced isomer quenching in the CaF$_2$ host, focusing on the effects of X-ray flux and temperature on the lifetime and yield of the isomer state. Our studies reveal a correlation between isomer production, isomer lifetime during irradiation, and post-irradiation afterglow of the target crystal across different temperatures, highlighting a strong relationship between isomer quenching and color-center dynamics. We developed a model to interpret the isomer quenching and the crystal's luminescence.

Publication Details

Journal
ArXiv.org
Published
2025-05-06
Primary Topic
Luminescence Properties of Advanced Materials
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article
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article

X-ray-induced quenching of the $^{229}$Th clock isomer in CaF$_2$

ArXiv.org
Luminescence Properties of Advanced Materials
article

X-ray-induced quenching of the $^{229}$Th clock isomer in CaF$_2$

article en

Abstract

Thorium-229 has the lowest nuclear-excited state (an isomer state) at approximately 8.356 eV, making it excitable with tabletop vacuum-ultraviolet lasers. Despite the recent success of laser excitation, the isomer quenching inside the solid-state environment remains unresolved. In this letter, we present experiments investigating X-ray-induced isomer quenching in the CaF$_2$ host, focusing on the effects of X-ray flux and temperature on the lifetime and yield of the isomer state. Our studies reveal a correlation between isomer production, isomer lifetime during irradiation, and post-irradiation afterglow of the target crystal across different temperatures, highlighting a strong relationship between isomer quenching and color-center dynamics. We developed a model to interpret the isomer quenching and the crystal's luminescence.

ArXiv.org
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Luminescence Properties of Advanced Materials
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X-ray-induced quenching of the $^{229}$Th clock isomer in CaF$_2$ · ArXiv.org (2025) | TGRS Research Map | TGRS