Plasmon-assisted photoelectron emission in a model cluster using time-dependent density functional theory and the time-dependent surface-flux method

We investigate plasmon-assisted photoelectron emission using a one-dimensional time-dependent density-functional theory (TDDFT) model. Photoelectron spectra are computed with the time-dependent surface-flux (t-SURFF) method. In addition to the expected above-threshold ionization (ATI) comb, we observe peaks that arise from long-lived plasmon oscillations and the associated electron emission occurring after the laser pulse. We further analyze the positions of these peaks and their scaling behavior with the laser intensity.

Publication Details

Journal
ArXiv.org
Published
2025-07-30
Primary Topic
Big Data and Digital Economy
Type
article
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article

Plasmon-assisted photoelectron emission in a model cluster using time-dependent density functional theory and the time-dependent surface-flux method

ArXiv.org
Big Data and Digital Economy
article

Plasmon-assisted photoelectron emission in a model cluster using time-dependent density functional theory and the time-dependent surface-flux method

article en

Abstract

We investigate plasmon-assisted photoelectron emission using a one-dimensional time-dependent density-functional theory (TDDFT) model. Photoelectron spectra are computed with the time-dependent surface-flux (t-SURFF) method. In addition to the expected above-threshold ionization (ATI) comb, we observe peaks that arise from long-lived plasmon oscillations and the associated electron emission occurring after the laser pulse. We further analyze the positions of these peaks and their scaling behavior with the laser intensity.

ArXiv.org
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Big Data and Digital Economy
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Plasmon-assisted photoelectron emission in a model cluster using time-dependent density functional theory and the time-dependent surface-flux method · ArXiv.org (2025) | TGRS Research Map | TGRS