Simple Fluctuations\nin Simple Glass Formers

Critical single-particle fluctuations associated with\nparticle\ndisplacements are inherent to simple glass-forming liquids in the\nlimit of large dimensions and leave a pseudocritical trace across\nall finite dimensions. This characteristic could serve as a crucial\ntest for distinguishing between theories of glass formation. We here\nexamine these critical fluctuations, as captured by the well-established\nnon-Gaussian parameter, within both mode-coupling theory (MCT) and\ndynamical mean-field theory (DMFT) across dimensions for hard sphere\nfluids and for the minimally structured Mari–Kurchan model.\nWe establish general scaling laws relevant to any liquid dynamics\ntheory in large dimensions and show that the dimensional scalings\npredicted by MCT are inconsistent with those from DMFT. Simulation\nresults for hard sphere fluids in moderately high dimensions align\nwith the DMFT scenario, reinforcing the relevance of mean-field theory\nfor capturing glass physics in finite dimensions. We identify potential\nadjustments to MCT to account for certain mean-field physics. Our\nfindings also highlight that local structure and spatial dimensionality\ncan affect single-particle critical fluctuations in nontrivial ways.

Publication Details

Journal
Figshare
Published
2024-11-26
DOI
https://doi.org/10.1021/acs.jpcb.4c05447.s001
Primary Topic
Wheat and Barley Genetics and Pathology
Type
article
Field-Weighted Citation Impact
0.00
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Simple Fluctuations\nin Simple Glass Formers

Figshare
Wheat and Barley Genetics and Pathology
article

Simple Fluctuations\nin Simple Glass Formers

article en

Abstract

Critical single-particle fluctuations associated with\nparticle\ndisplacements are inherent to simple glass-forming liquids in the\nlimit of large dimensions and leave a pseudocritical trace across\nall finite dimensions. This characteristic could serve as a crucial\ntest for distinguishing between theories of glass formation. We here\nexamine these critical fluctuations, as captured by the well-established\nnon-Gaussian parameter, within both mode-coupling theory (MCT) and\ndynamical mean-field theory (DMFT) across dimensions for hard sphere\nfluids and for the minimally structured Mari–Kurchan model.\nWe establish general scaling laws relevant to any liquid dynamics\ntheory in large dimensions and show that the dimensional scalings\npredicted by MCT are inconsistent with those from DMFT. Simulation\nresults for hard sphere fluids in moderately high dimensions align\nwith the DMFT scenario, reinforcing the relevance of mean-field theory\nfor capturing glass physics in finite dimensions. We identify potential\nadjustments to MCT to account for certain mean-field physics. Our\nfindings also highlight that local structure and spatial dimensionality\ncan affect single-particle critical fluctuations in nontrivial ways.

Figshare
Openalex Percentile: Top 38%
Wheat and Barley Genetics and Pathology
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.

Simple Fluctuations\nin Simple Glass Formers · Figshare (2024) | TGRS Research Map | TGRS