Superradiance of strongly interacting dipolar excitons in moiré quantum materials

Moiré lattices created in two-dimensional heterostructures exhibit rich many-body physics of interacting electrons and excitons and, at the same time, suggest promising optoelectronic applications. Here, we study the cooperative radiance of moiré excitons that is demonstrated to emerge from the deep subwavelength nature of the moiré lattice and the strong excitonic onsite interaction. In particular, we show that the static dipole-dipole interaction between interlayer excitons can strongly affect their cooperative optical properties, suppressing superradiance of disordered states while enhancing superradiance of ordered phases of moiré excitons. Moreover, we show that doping permits direct control of optical cooperativity, e.g., by generating supperradiant dynamics of otherwise subradiant states of excitons. Our results show that interlayer moiré excitons offer a unique platform for exploring cooperative optical phenomena in strongly interacting many-body systems, thus, holding promise for applications in quantum nonlinear optics.

Publication Details

Journal
reposiTUm (TU Wien)
Published
2024-10-11
DOI
https://doi.org/10.34726/8686
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
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article

Superradiance of strongly interacting dipolar excitons in moiré quantum materials

reposiTUm (TU Wien)
Strong Light-Matter Interactions
article

Superradiance of strongly interacting dipolar excitons in moiré quantum materials

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Abstract

Moiré lattices created in two-dimensional heterostructures exhibit rich many-body physics of interacting electrons and excitons and, at the same time, suggest promising optoelectronic applications. Here, we study the cooperative radiance of moiré excitons that is demonstrated to emerge from the deep subwavelength nature of the moiré lattice and the strong excitonic onsite interaction. In particular, we show that the static dipole-dipole interaction between interlayer excitons can strongly affect their cooperative optical properties, suppressing superradiance of disordered states while enhancing superradiance of ordered phases of moiré excitons. Moreover, we show that doping permits direct control of optical cooperativity, e.g., by generating supperradiant dynamics of otherwise subradiant states of excitons. Our results show that interlayer moiré excitons offer a unique platform for exploring cooperative optical phenomena in strongly interacting many-body systems, thus, holding promise for applications in quantum nonlinear optics.

reposiTUm (TU Wien)
Openalex Percentile: Top 69%
Strong Light-Matter Interactions
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