Ultrafast Dual\nActivation of C(sp<sup>3</sup>)–H\nand C(sp<sup>2</sup>)–H Bonds in an Arc Plasma-Initiated Microdroplet

This study demonstrates a method that utilizes arc plasma-induced\nmicrodroplet reactions to synthesize dual-activated products with\nC(sp<sup>3</sup>)–N and C(sp<sup>2</sup>)–O bonds starting\nfrom C–H bonds. This innovative process utilizes arc- and microdroplet-generated\nhydroxyl radicals and water dimer radical cations, opening new possibilities\nfor the multisite derivatization of small molecules.

Publication Details

Journal
Figshare
Published
2024-11-19
DOI
https://doi.org/10.1021/acs.orglett.4c03782.s001
Primary Topic
Radical Photochemical Reactions
Type
article
Field-Weighted Citation Impact
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article

Ultrafast Dual\nActivation of C(sp3)–H\nand C(sp2)–H Bonds in an Arc Plasma-Initiated Microdroplet

Figshare
Radical Photochemical Reactions
article

Ultrafast Dual\nActivation of C(sp3)–H\nand C(sp2)–H Bonds in an Arc Plasma-Initiated Microdroplet

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Abstract

This study demonstrates a method that utilizes arc plasma-induced\nmicrodroplet reactions to synthesize dual-activated products with\nC(sp<sup>3</sup>)–N and C(sp<sup>2</sup>)–O bonds starting\nfrom C–H bonds. This innovative process utilizes arc- and microdroplet-generated\nhydroxyl radicals and water dimer radical cations, opening new possibilities\nfor the multisite derivatization of small molecules.

Figshare
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Radical Photochemical Reactions
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Ultrafast Dual\nActivation of C(sp<sup>3</sup>)–H\nand C(sp<sup>2</sup>)–H Bonds in an Arc Plasma-Initiated Microdroplet · Figshare (2024) | TGRS Research Map | TGRS