Fully Stretchableand Self-Healing Graphene-HydrogelE‑Skin with Temperature-Strain Self-Calibration

Hydrogels exhibit mechanical properties very similar to biological skin, rendering them promising candidates for electronic skin (e-skin) sensors. However, these materials suffer from significant temperature-induced electrical drift and unstable interfacial contact with metallic electrodes. In this study, we employ elastic graphene foam as electrodes to realize a fully flexible hydrogel device architecture. By designing straight-line and serpentine hydrogel geometries, we enable temperature self-calibration during strain measurements. The resulting hydrogel sensor demonstrates exceptional performance, including constant strain sensitivity (GF = 2.44 with linearity <i>R</i><sup>2</sup> = 0.9999), rapid strain dynamic response (70 ms), low strain detection limit (0.05%), and low temperature drift. This approach not only addresses critical limitations in hydrogel-based sensing platforms but also establishes a robust framework for developing more reliable and versatile flexible sensors.

Publication Details

Journal
Figshare
Published
2025-02-05
DOI
https://doi.org/10.1021/acsanm.4c06895.s001
Primary Topic
Advanced Sensor and Energy Harvesting Materials
Type
article
Field-Weighted Citation Impact
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article

Fully Stretchableand Self-Healing Graphene-HydrogelE‑Skin with Temperature-Strain Self-Calibration

Figshare
Advanced Sensor and Energy Harvesting Materials
article

Fully Stretchableand Self-Healing Graphene-HydrogelE‑Skin with Temperature-Strain Self-Calibration

article en

Abstract

Hydrogels exhibit mechanical properties very similar to biological skin, rendering them promising candidates for electronic skin (e-skin) sensors. However, these materials suffer from significant temperature-induced electrical drift and unstable interfacial contact with metallic electrodes. In this study, we employ elastic graphene foam as electrodes to realize a fully flexible hydrogel device architecture. By designing straight-line and serpentine hydrogel geometries, we enable temperature self-calibration during strain measurements. The resulting hydrogel sensor demonstrates exceptional performance, including constant strain sensitivity (GF = 2.44 with linearity <i>R</i><sup>2</sup> = 0.9999), rapid strain dynamic response (70 ms), low strain detection limit (0.05%), and low temperature drift. This approach not only addresses critical limitations in hydrogel-based sensing platforms but also establishes a robust framework for developing more reliable and versatile flexible sensors.

Figshare
Openalex Percentile: Top 58%
Advanced Sensor and Energy Harvesting Materials
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