TopologicallyEngineered High‑<i>Q</i> Quasi-BIC Metasurfaces forEnhanced Near-Infrared Emission in PbSQuantum Dots

Enhancing photoluminescence (PL) efficiency in colloidal quantum dots is pivotal for next-generation near-infrared photodetectors, imaging systems, and photonic devices. Conventional methods, especially metal-based plasmonic structures, suffer from large optical losses, which limits their practical use. Here, we introduce a quasi-bound state in the continuum (quasi-BIC) metasurface on a silicon-on-insulator platform, tailored to provide high-quality factor resonances with minimized losses. Utilizing topological charge engineering and controlled in-plane asymmetry in silicon cylinder arrays, we developed a robust quasi-BIC capable of maintaining a high <i>Q</i> factor across a broad angular range, achieving an experimental <i>Q</i> factor of 3031 at normal incidence. This approach significantly enhances near-field interactions, achieving a ≤110-fold increase in PL for PbS quantum dots at 33 K and a 41-fold enhancement at room temperature. Our findings offer a scalable, cost-effective solution for enhancing light emission in advanced optoelectronic applications.

Publication Details

Journal
Figshare
Published
2025-01-15
DOI
https://doi.org/10.1021/acs.nanolett.4c05710.s001
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
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article

TopologicallyEngineered High‑Q Quasi-BIC Metasurfaces forEnhanced Near-Infrared Emission in PbSQuantum Dots

Figshare
Plasmonic and Surface Plasmon Research
article

TopologicallyEngineered High‑Q Quasi-BIC Metasurfaces forEnhanced Near-Infrared Emission in PbSQuantum Dots

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Abstract

Enhancing photoluminescence (PL) efficiency in colloidal quantum dots is pivotal for next-generation near-infrared photodetectors, imaging systems, and photonic devices. Conventional methods, especially metal-based plasmonic structures, suffer from large optical losses, which limits their practical use. Here, we introduce a quasi-bound state in the continuum (quasi-BIC) metasurface on a silicon-on-insulator platform, tailored to provide high-quality factor resonances with minimized losses. Utilizing topological charge engineering and controlled in-plane asymmetry in silicon cylinder arrays, we developed a robust quasi-BIC capable of maintaining a high <i>Q</i> factor across a broad angular range, achieving an experimental <i>Q</i> factor of 3031 at normal incidence. This approach significantly enhances near-field interactions, achieving a ≤110-fold increase in PL for PbS quantum dots at 33 K and a 41-fold enhancement at room temperature. Our findings offer a scalable, cost-effective solution for enhancing light emission in advanced optoelectronic applications.

Figshare
Openalex Percentile: Top 58%
Plasmonic and Surface Plasmon Research
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