Superconductivity Induced by Strong Electron-Exciton Coupling in Doped Atomically Thin Semiconductor Heterostructures

We study a mechanism to induce superconductivity in atomically thin semiconductors where excitons mediate an effective attraction between electrons. Our model includes interaction effects beyond the paradigm of phonon-mediated superconductivity and connects to the well-established limits of Bose and Fermi polarons. By accounting for the strong-coupling physics of trions, we find that the effective electron-exciton interaction develops a strong frequency and momentum dependence accompanied by the system undergoing an emerging BCS-BEC crossover from weakly bound s-wave Cooper pairs to a superfluid of bipolarons. Even at strong-coupling the bipolarons remain relatively light, resulting in critical temperatures of up to 10% of the Fermi temperature. This renders heterostructures of two-dimensional materials a promising candidate to realize superconductivity at high critical temperatures set by electron doping and trion binding energies.

Publication Details

Journal
Repository for Publications and Research Data (ETH Zurich)
Published
2024-11-27
DOI
https://doi.org/10.3929/ethz-b-000708017
Primary Topic
Electronic and Structural Properties of Oxides
Type
article
Field-Weighted Citation Impact
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article

Superconductivity Induced by Strong Electron-Exciton Coupling in Doped Atomically Thin Semiconductor Heterostructures

Repository for Publications and Research Data (ETH Zurich)
Electronic and Structural Properties of Oxides
article

Superconductivity Induced by Strong Electron-Exciton Coupling in Doped Atomically Thin Semiconductor Heterostructures

article en

Abstract

We study a mechanism to induce superconductivity in atomically thin semiconductors where excitons mediate an effective attraction between electrons. Our model includes interaction effects beyond the paradigm of phonon-mediated superconductivity and connects to the well-established limits of Bose and Fermi polarons. By accounting for the strong-coupling physics of trions, we find that the effective electron-exciton interaction develops a strong frequency and momentum dependence accompanied by the system undergoing an emerging BCS-BEC crossover from weakly bound s-wave Cooper pairs to a superfluid of bipolarons. Even at strong-coupling the bipolarons remain relatively light, resulting in critical temperatures of up to 10% of the Fermi temperature. This renders heterostructures of two-dimensional materials a promising candidate to realize superconductivity at high critical temperatures set by electron doping and trion binding energies.

Repository for Publications and Research Data (ETH Zurich)
Openalex Percentile: Top 80%
Electronic and Structural Properties of Oxides
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