Femtosecond electron dynamics driven by ponderomotive gradients

Electrons driven by the oscillating electric field of intense femtosecond laser pulses experience an effective cycle-averaged ponderomotive potential. This thesis investigates the ponderomotive effects of circularly polarized few-cycle pulses and standing waves on photoionization, photoemission, and the subsequent electron motion. Reconstructing the time-dependent dipole moment of recolliding electron wave packets from an extreme ultraviolet absorption spectrum reveals an envelope-driven recollision channel in circularly polarized light, as predicted by the theory of recolliding periodic orbits. Furthermore, tomography of photoelectron angular distributions is achieved using velocity-map imaging within a femtosecond enhancement cavity operating at 100MHz. This cavity supports two counter-propagating pulses that form a transient standing wave at the focus. Exploiting the standing wave structure allows to probe the photoemission at different crystal facets of a tungsten nanotip and to minimize the source volume of above-threshold ionization. In addition, the high-intensity Kapitza-Dirac effect for resonantly ionized electrons in the picosecond regime is presented together with still unexplained diffraction results for femtosecond pulses. The intense intra-cavity standing waves are a promising tool for coherent control of electron matter waves, potentially advancing the development of a femtosecond electron interferometer at low energies.

Publication Details

Journal
heiDOK (Heidelberg University)
Published
2025-01-01
DOI
https://doi.org/10.11588/heidok.00036534
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
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article

Femtosecond electron dynamics driven by ponderomotive gradients

heiDOK (Heidelberg University)
Laser-Matter Interactions and Applications
article

Femtosecond electron dynamics driven by ponderomotive gradients

article en

Abstract

Electrons driven by the oscillating electric field of intense femtosecond laser pulses experience an effective cycle-averaged ponderomotive potential. This thesis investigates the ponderomotive effects of circularly polarized few-cycle pulses and standing waves on photoionization, photoemission, and the subsequent electron motion. Reconstructing the time-dependent dipole moment of recolliding electron wave packets from an extreme ultraviolet absorption spectrum reveals an envelope-driven recollision channel in circularly polarized light, as predicted by the theory of recolliding periodic orbits. Furthermore, tomography of photoelectron angular distributions is achieved using velocity-map imaging within a femtosecond enhancement cavity operating at 100MHz. This cavity supports two counter-propagating pulses that form a transient standing wave at the focus. Exploiting the standing wave structure allows to probe the photoemission at different crystal facets of a tungsten nanotip and to minimize the source volume of above-threshold ionization. In addition, the high-intensity Kapitza-Dirac effect for resonantly ionized electrons in the picosecond regime is presented together with still unexplained diffraction results for femtosecond pulses. The intense intra-cavity standing waves are a promising tool for coherent control of electron matter waves, potentially advancing the development of a femtosecond electron interferometer at low energies.

heiDOK (Heidelberg University)
Openalex Percentile: Top 66%
Laser-Matter Interactions and Applications
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