Sulfoximine\nAided Ru(II)-Catalyzed Asymmetric Double\nC(sp<sup>2</sup>)–H Hydroarylations of Olefins

Presented here is a sulfoximine-directed Ru(II)-catalyzed\nasymmetric\nintramolecular double C(sp<sup>2</sup>)–H hydroarylation of\nolefins. This process provides a diastereoselective and enantiospecific\nsynthetic route to highly substituted tetrahydrobenzodifurans. Notably,\nthe reaction accommodates labile functional groups and is scalable\nto gram quantities.

Publication Details

Journal
Figshare
Published
2024-10-21
DOI
https://doi.org/10.1021/acs.orglett.4c03524.s001
Primary Topic
Catalytic C–H Functionalization Methods
Type
article
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Sulfoximine\nAided Ru(II)-Catalyzed Asymmetric Double\nC(sp2)–H Hydroarylations of Olefins

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Catalytic C–H Functionalization Methods
article

Sulfoximine\nAided Ru(II)-Catalyzed Asymmetric Double\nC(sp2)–H Hydroarylations of Olefins

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Abstract

Presented here is a sulfoximine-directed Ru(II)-catalyzed\nasymmetric\nintramolecular double C(sp<sup>2</sup>)–H hydroarylation of\nolefins. This process provides a diastereoselective and enantiospecific\nsynthetic route to highly substituted tetrahydrobenzodifurans. Notably,\nthe reaction accommodates labile functional groups and is scalable\nto gram quantities.

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Catalytic C–H Functionalization Methods
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Sulfoximine\nAided Ru(II)-Catalyzed Asymmetric Double\nC(sp<sup>2</sup>)–H Hydroarylations of Olefins · Figshare (2024) | TGRS Research Map | TGRS