Spin-ValveEffect in Junctions with a Single Ferromagnet

Spin valves are essential components in spintronic memory devices whose conductance is modulated by controlling spin-polarized electron tunnelling through the alignment of the magnetization in ferromagnetic elements. Whereas conventional spin valves unavoidably require at least two ferromagnetic elements, here we demonstrate a van der Waals spin valve based on a tunnel junction that comprises only one such ferromagnetic layer. Our devices combine an Fe<sub>3</sub>GeTe<sub>2</sub> electrode acting as a spin injector together with a paramagnetic tunnel barrier, formed by a CrBr<sub>3</sub> multilayer operated above its Curie temperature. We show that these devices exhibit a conductance modulation with values comparable to those of conventional spin valves. A quantitative analysis of the magnetoconductance that accounts for the field-induced magnetization of CrBr<sub>3</sub>, including the effect of exchange interaction, confirms that the spin valve effect originates from the paramagnetic response of the barrier, in the absence of spontaneous magnetization in CrBr<sub>3</sub>.

Publication Details

Journal
Figshare
Published
2025-02-19
DOI
https://doi.org/10.1021/acs.nanolett.4c06301.s001
Primary Topic
Magnetic properties of thin films
Type
article
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article

Spin-ValveEffect in Junctions with a Single Ferromagnet

Figshare
Magnetic properties of thin films
article

Spin-ValveEffect in Junctions with a Single Ferromagnet

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Abstract

Spin valves are essential components in spintronic memory devices whose conductance is modulated by controlling spin-polarized electron tunnelling through the alignment of the magnetization in ferromagnetic elements. Whereas conventional spin valves unavoidably require at least two ferromagnetic elements, here we demonstrate a van der Waals spin valve based on a tunnel junction that comprises only one such ferromagnetic layer. Our devices combine an Fe<sub>3</sub>GeTe<sub>2</sub> electrode acting as a spin injector together with a paramagnetic tunnel barrier, formed by a CrBr<sub>3</sub> multilayer operated above its Curie temperature. We show that these devices exhibit a conductance modulation with values comparable to those of conventional spin valves. A quantitative analysis of the magnetoconductance that accounts for the field-induced magnetization of CrBr<sub>3</sub>, including the effect of exchange interaction, confirms that the spin valve effect originates from the paramagnetic response of the barrier, in the absence of spontaneous magnetization in CrBr<sub>3</sub>.

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Magnetic properties of thin films
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