Multiple HyperbolicDispersion Branches and BroadbandCanalization in a Phonon-Polaritonic Heterostructure

Hyperbolic polaritons in anisotropic crystals hold great promise for guiding the flow of light at deep-subwavelength scales. However, conventional hyperbolic dispersion with a single pair of symmetric branches inherently confines polaritons to propagate only within specific spatial directions. Here we demonstrate a multibranch in-plane hyperbolic dispersion in a phonon-polaritonic heterostructure composed of α-phase molybdenum trioxide (α-MoO<sub>3</sub>) and 4H-silicon carbide (4H-SiC). Leveraging the in-plane hyperbolicity of α-MoO<sub>3</sub> and the interlayer coupling with 4H-SiC, the polaritons manifest distinct dispersive responses along the mutually orthogonal crystal directions of α-MoO<sub>3</sub>, enabling asymmetric multidirectional polariton propagation. Furthermore, the dispersion contours of polaritons along the [100] crystal direction of α-MoO<sub>3</sub> evolves into flat bands as the frequency decreases, yielding broadband polariton canalization in the low-frequency region. These findings deepen our understanding of the evolution of polariton dispersions in α-MoO<sub>3</sub>/4H-SiC heterostructures and highlight the potential of this phonon-polaritonic heterostructure as a versatile platform for nanolight manipulation.

Publication Details

Journal
Figshare
Published
2025-02-07
DOI
https://doi.org/10.1021/acs.nanolett.4c04633.s001
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
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article

Multiple HyperbolicDispersion Branches and BroadbandCanalization in a Phonon-Polaritonic Heterostructure

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Plasmonic and Surface Plasmon Research
article

Multiple HyperbolicDispersion Branches and BroadbandCanalization in a Phonon-Polaritonic Heterostructure

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Abstract

Hyperbolic polaritons in anisotropic crystals hold great promise for guiding the flow of light at deep-subwavelength scales. However, conventional hyperbolic dispersion with a single pair of symmetric branches inherently confines polaritons to propagate only within specific spatial directions. Here we demonstrate a multibranch in-plane hyperbolic dispersion in a phonon-polaritonic heterostructure composed of α-phase molybdenum trioxide (α-MoO<sub>3</sub>) and 4H-silicon carbide (4H-SiC). Leveraging the in-plane hyperbolicity of α-MoO<sub>3</sub> and the interlayer coupling with 4H-SiC, the polaritons manifest distinct dispersive responses along the mutually orthogonal crystal directions of α-MoO<sub>3</sub>, enabling asymmetric multidirectional polariton propagation. Furthermore, the dispersion contours of polaritons along the [100] crystal direction of α-MoO<sub>3</sub> evolves into flat bands as the frequency decreases, yielding broadband polariton canalization in the low-frequency region. These findings deepen our understanding of the evolution of polariton dispersions in α-MoO<sub>3</sub>/4H-SiC heterostructures and highlight the potential of this phonon-polaritonic heterostructure as a versatile platform for nanolight manipulation.

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Plasmonic and Surface Plasmon Research
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