Metallic Electro-opticEffect in Gapped Bilayer Graphene

Electro-optic (EO) modulation is a critical device action in photonics. Recently, the non-Drude dynamics induced by the Berry curvature dipole (BCD) in metals have attracted attention as a potential candidate for terahertz EO modulation. However, such BCD-induced EO effects can be challenging to realize, often requiring flat bands and complex materials such as a strained magic-angle twisted bilayer graphene on hexagonal boron nitride. Here, we argue that metallic EO can be achieved with a much simpler material, gapped bilayer graphene, with EO coefficients comparable to that in flat-band materials in the terahertz range. In particular, we find metallic EO can be realized <i>without</i> a Berry curvature dipole; we identify skew-scattering and a “snap” (third-order derivative of velocity) can readily produce pronounced Pockels and Kerr EO effects in clean metals. These yield nonreciprocal and field-activated birefringence and field-induced modulations to transmission and reflection, essential components for terahertz EO modulators.

Publication Details

Journal
Figshare
Published
2025-01-15
DOI
https://doi.org/10.1021/acs.nanolett.4c03771.s001
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
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article

Metallic Electro-opticEffect in Gapped Bilayer Graphene

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Plasmonic and Surface Plasmon Research
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Metallic Electro-opticEffect in Gapped Bilayer Graphene

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Abstract

Electro-optic (EO) modulation is a critical device action in photonics. Recently, the non-Drude dynamics induced by the Berry curvature dipole (BCD) in metals have attracted attention as a potential candidate for terahertz EO modulation. However, such BCD-induced EO effects can be challenging to realize, often requiring flat bands and complex materials such as a strained magic-angle twisted bilayer graphene on hexagonal boron nitride. Here, we argue that metallic EO can be achieved with a much simpler material, gapped bilayer graphene, with EO coefficients comparable to that in flat-band materials in the terahertz range. In particular, we find metallic EO can be realized <i>without</i> a Berry curvature dipole; we identify skew-scattering and a “snap” (third-order derivative of velocity) can readily produce pronounced Pockels and Kerr EO effects in clean metals. These yield nonreciprocal and field-activated birefringence and field-induced modulations to transmission and reflection, essential components for terahertz EO modulators.

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Plasmonic and Surface Plasmon Research
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