C–H Arylationof Aminoquinones through ElectrochemicalDenitrogenative Coupling

An electrooxidative C–C coupling between arylhydrazines and aminoquinones has been developed for the construction of aryl-substituted aminoquinones, which features excellent chemo- and regioselectivity. Mechanistic studies support the idea that the denitrogenative formation of aryl radicals might be involved in the metal-free C–H arylation.

Publication Details

Journal
Figshare
Published
2025-02-05
DOI
https://doi.org/10.1021/acs.joc.4c02909.s001
Primary Topic
Radical Photochemical Reactions
Type
article
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article

C–H Arylationof Aminoquinones through ElectrochemicalDenitrogenative Coupling

Figshare
Radical Photochemical Reactions
article

C–H Arylationof Aminoquinones through ElectrochemicalDenitrogenative Coupling

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Abstract

An electrooxidative C–C coupling between arylhydrazines and aminoquinones has been developed for the construction of aryl-substituted aminoquinones, which features excellent chemo- and regioselectivity. Mechanistic studies support the idea that the denitrogenative formation of aryl radicals might be involved in the metal-free C–H arylation.

Figshare
Clean water and sanitation
Openalex Percentile: Top 69%
Radical Photochemical Reactions
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C–H Arylationof Aminoquinones through ElectrochemicalDenitrogenative Coupling · Figshare (2025) | TGRS Research Map | TGRS