Contrasting magnetic behavior in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>MnSc</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>X</mml:mi> <mml:mn>4</mml:mn> </mml:msub> </mml:mrow> </mml:math>
The spinel compounds ${\mathrm{MnSc}}_{2}{X}_{4}$ are highly frustrated and candidate materials for vortex-like 3 q magnetic states, such as skyrmions, with propagation vectors in the [111] plane. Because of the strong magnetoelastic coupling, we could extract a refined magnetic $(H,T)$ phase diagram for ${\mathrm{MnSc}}_{2}{\mathrm{S}}_{4}$ from ultrasound and dilatometry measurements. We found a variety of magnetic phases, including the skyrmion phase, which is stable down to lowest temperatures. In comparison, we investigated ${\mathrm{MnSc}}_{2}{\mathrm{Se}}_{4}$, having a larger distance between the magnetic ${\mathrm{Mn}}^{3+}$ ions using the same methods. Unlike in ${\mathrm{MnSc}}_{2}{\mathrm{S}}_{4}$, we found no skyrmion phase and overall a lack of sharp anomalies indicative of phase transitions, neither in dilatometry nor ultrasound nor in specific heat and ac-susceptibility data. Motivated by our findings, we performed model calculations, which reproduced the experimentally observed magnetostriction and specific-heat results reasonably well.
Authors
- Tino Gottschall (ORCID: https://orcid.org/0000-0002-4117-8169)
- Mahmoud Deeb
- A. Hauspurg
- M. Doerr (ORCID: https://orcid.org/0000-0002-5916-6756)
- Atsuhiko Miyata (ORCID: https://orcid.org/0000-0002-1726-0314)
- Hidemaro Suwa (ORCID: https://orcid.org/0000-0002-6026-2630)
- S. Zherlitsyn
- J. Wosnitza (ORCID: https://orcid.org/0009-0008-4136-5643)
- V. Tsurkan
- Sergey Granovsky (ORCID: https://orcid.org/0000-0001-9425-6696)
- M. Rotter (ORCID: https://orcid.org/0000-0001-6779-179X)
- L. Prodan
- S. Chattopadhyay (ORCID: https://orcid.org/0000-0001-9061-2139)
- Justus Grumbach
- J. Sourd
Institutions
- University of Augsburg (DE)
- Helmholtz-Zentrum Dresden-Rossendorf (DE)
- The University of Tokyo (JP)
- Technische Universität Dresden (DE)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-21
- DOI
- https://doi.org/10.1103/479d-4jvy
- Primary Topic
- Magnetic and transport properties of perovskites and related materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Agenția Națională pentru Cercetare și Dezvoltare
- Deutsche Forschungsgemeinschaft
- Helmholtz-Zentrum Dresden-Rossendorf
- Japan Society for the Promotion of Science