Contrasting magnetic behavior in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>MnSc</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>X</mml:mi> <mml:mn>4</mml:mn> </mml:msub> </mml:mrow> </mml:math>

The spinel compounds ${\mathrm{MnSc}}_{2}{X}_{4}$ are highly frustrated and candidate materials for vortex-like 3 q magnetic states, such as skyrmions, with propagation vectors in the [111] plane. Because of the strong magnetoelastic coupling, we could extract a refined magnetic $(H,T)$ phase diagram for ${\mathrm{MnSc}}_{2}{\mathrm{S}}_{4}$ from ultrasound and dilatometry measurements. We found a variety of magnetic phases, including the skyrmion phase, which is stable down to lowest temperatures. In comparison, we investigated ${\mathrm{MnSc}}_{2}{\mathrm{Se}}_{4}$, having a larger distance between the magnetic ${\mathrm{Mn}}^{3+}$ ions using the same methods. Unlike in ${\mathrm{MnSc}}_{2}{\mathrm{S}}_{4}$, we found no skyrmion phase and overall a lack of sharp anomalies indicative of phase transitions, neither in dilatometry nor ultrasound nor in specific heat and ac-susceptibility data. Motivated by our findings, we performed model calculations, which reproduced the experimentally observed magnetostriction and specific-heat results reasonably well.

Authors

Institutions

Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-21
DOI
https://doi.org/10.1103/479d-4jvy
Primary Topic
Magnetic and transport properties of perovskites and related materials
Type
article
Field-Weighted Citation Impact
0.00

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Contrasting magnetic behavior in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>MnSc</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>X</mml:mi> <mml:mn>4</mml:mn> </mml:msub> </mml:mrow> </mml:math>

Tino Gottschall, Mahmoud Deeb, A. Hauspurg, M. Doerr et al.
Physical review. B./Physical review. B
Magnetic and transport properties of perovskites and related materials
article

Contrasting magnetic behavior in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>MnSc</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>X</mml:mi> <mml:mn>4</mml:mn> </mml:msub> </mml:mrow> </mml:math>

Tino Gottschall, Mahmoud Deeb, A. Hauspurg, M. Doerr, Atsuhiko Miyata, Hidemaro Suwa, S. Zherlitsyn, J. Wosnitza, V. Tsurkan, Sergey Granovsky, M. Rotter, L. Prodan, S. Chattopadhyay, Justus Grumbach, J. Sourd
article en

Abstract

The spinel compounds ${\mathrm{MnSc}}_{2}{X}_{4}$ are highly frustrated and candidate materials for vortex-like 3 q magnetic states, such as skyrmions, with propagation vectors in the [111] plane. Because of the strong magnetoelastic coupling, we could extract a refined magnetic $(H,T)$ phase diagram for ${\mathrm{MnSc}}_{2}{\mathrm{S}}_{4}$ from ultrasound and dilatometry measurements. We found a variety of magnetic phases, including the skyrmion phase, which is stable down to lowest temperatures. In comparison, we investigated ${\mathrm{MnSc}}_{2}{\mathrm{Se}}_{4}$, having a larger distance between the magnetic ${\mathrm{Mn}}^{3+}$ ions using the same methods. Unlike in ${\mathrm{MnSc}}_{2}{\mathrm{S}}_{4}$, we found no skyrmion phase and overall a lack of sharp anomalies indicative of phase transitions, neither in dilatometry nor ultrasound nor in specific heat and ac-susceptibility data. Motivated by our findings, we performed model calculations, which reproduced the experimentally observed magnetostriction and specific-heat results reasonably well.

Physical review. B./Physical review. BVol. 112(21)
University of Augsburg (DE), Helmholtz-Zentrum Dresden-Rossendorf (DE), The University of Tokyo (JP), Technische Universität Dresden (DE)
Agenția Națională pentru Cercetare și Dezvoltare, Deutsche Forschungsgemeinschaft, Helmholtz-Zentrum Dresden-Rossendorf, Japan Society for the Promotion of Science
Openalex Percentile: Top 70%
Magnetic and transport properties of perovskites and related materials
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.