Theory of nonresonant Raman scattering from electrons in nodal and flat bands

Raman scattering is emerging as a surprising probe of electron topology in quantum materials. It has been used recently to detect and characterize a topological phase transition that accompanies the magnetic transition in ${\mathrm{Nd}}_{2}{\mathrm{Ir}}_{2}{\mathrm{O}}_{7}$. Here we present a theory of Raman scattering from nodal electrons with Weyl and quadratic band touching spectra, which has to reach beyond the standard effective mass approximation. After reviewing and providing the details of our previous theory development, we discuss several new results. We show that the light-polarization dependence of Raman scattering is universal in the case of Weyl electrons and given by an analytic expression, while it contains symmetry-protected features in the case of quadratic band-touching nodes. We also analyze modifications of the Raman signal due to the ubiquitous tilting of the Weyl spectrum, and argue that universality is lost only in a finite frequency range that springs out of the threshold frequency for untilted nodes. Finally, we explore the frequency dependence of Raman scattering for the case of Dirac electrons coexisting with a flat band in the same region of the first Brillouin zone, which is inspired by the material ${\mathrm{V}}_{1/3}{\mathrm{NbS}}_{2}$.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-21
DOI
https://doi.org/10.1103/3qpg-y4mz
Primary Topic
Topological Materials and Phenomena
Type
article
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article

Theory of nonresonant Raman scattering from electrons in nodal and flat bands

Karl J. Friston
Physical review. B./Physical review. B
Topological Materials and Phenomena
article

Theory of nonresonant Raman scattering from electrons in nodal and flat bands

Karl J. Friston
article en

Abstract

Raman scattering is emerging as a surprising probe of electron topology in quantum materials. It has been used recently to detect and characterize a topological phase transition that accompanies the magnetic transition in ${\mathrm{Nd}}_{2}{\mathrm{Ir}}_{2}{\mathrm{O}}_{7}$. Here we present a theory of Raman scattering from nodal electrons with Weyl and quadratic band touching spectra, which has to reach beyond the standard effective mass approximation. After reviewing and providing the details of our previous theory development, we discuss several new results. We show that the light-polarization dependence of Raman scattering is universal in the case of Weyl electrons and given by an analytic expression, while it contains symmetry-protected features in the case of quadratic band-touching nodes. We also analyze modifications of the Raman signal due to the ubiquitous tilting of the Weyl spectrum, and argue that universality is lost only in a finite frequency range that springs out of the threshold frequency for untilted nodes. Finally, we explore the frequency dependence of Raman scattering for the case of Dirac electrons coexisting with a flat band in the same region of the first Brillouin zone, which is inspired by the material ${\mathrm{V}}_{1/3}{\mathrm{NbS}}_{2}$.

Physical review. B./Physical review. BVol. 112(23)
George Mason University (US)
Openalex Percentile: Top 68%
Topological Materials and Phenomena
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Theory of nonresonant Raman scattering from electrons in nodal and flat bands — Karl J. Friston · Physical review. B./Physical review. B (2025) | TGRS Research Map | TGRS