Phonons in Epitaxial <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>DySi</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> : From th

Using nuclear inelastic scattering on ^{161}Dy, we determined the Dy-partial phonon density of states of epitaxial DySi_{2} in bulk and self-organized nanoislands and nanowires (NWs) on vicinal Si(001) surface. Compared to the bulk, the nanoislands exhibit softening of the crystal lattice, which is further enhanced in the NWs and significantly affects their thermodynamic and elastic properties. Our ab initio calculations reveal that the origin of this effect is the vibrations of Dy atoms located at the surfaces of the nanoislands and the NWs as well as forming a (2×4) reconstruction on the Si(001) surface between the NWs. The results demonstrate that, opposite to the widely accepted anisotropic lattice mismatch model, the NWs form with their length along the [0001] direction of the strained hexagonal unit cell with lattice parameters close to the Si(001) surface.

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Publication Details

Journal
Physical Review Letters
Published
2025-11-20
DOI
https://doi.org/10.1103/4r3t-tr77
Primary Topic
Semiconductor materials and interfaces
Type
article
Field-Weighted Citation Impact
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article

Phonons in Epitaxial <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>DySi</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> : From th

Karl J. Friston
Physical Review Letters
Semiconductor materials and interfaces
article

Phonons in Epitaxial <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>DySi</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> : From th

Karl J. Friston
article en

Abstract

Using nuclear inelastic scattering on ^{161}Dy, we determined the Dy-partial phonon density of states of epitaxial DySi_{2} in bulk and self-organized nanoislands and nanowires (NWs) on vicinal Si(001) surface. Compared to the bulk, the nanoislands exhibit softening of the crystal lattice, which is further enhanced in the NWs and significantly affects their thermodynamic and elastic properties. Our ab initio calculations reveal that the origin of this effect is the vibrations of Dy atoms located at the surfaces of the nanoislands and the NWs as well as forming a (2×4) reconstruction on the Si(001) surface between the NWs. The results demonstrate that, opposite to the widely accepted anisotropic lattice mismatch model, the NWs form with their length along the [0001] direction of the strained hexagonal unit cell with lattice parameters close to the Si(001) surface.

Physical Review LettersVol. 135(25)
Karlsruhe Institute of Technology (DE), European Synchrotron Radiation Facility (FR), Institute of Nuclear Physics, Polish Academy of Sciences (PL), HUN-REN Wigner Research Centre for Physics (HU)
Openalex Percentile: Top 68%
Semiconductor materials and interfaces
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