Bidirectional Ultrafast Control of Charge Density Waves via Phase Competition

The intricate competition between coexisting charge density waves (CDWs) can lead to rich phenomena, offering unique opportunities for phase manipulation through electromagnetic stimuli. Leveraging time-resolved x-ray diffraction, we demonstrate ultrafast control of a CDW in EuTe_{4} upon optical excitation. At low excitation intensities, the amplitude of one of the coexisting CDW orders increases at the expense of the competing CDW, whereas at high intensities, it exhibits a nonmonotonic temporal evolution characterized by both enhancement and reduction. This transient bidirectional controllability, tunable by adjusting photoexcitation intensity, arises from the interplay between optical quenching and phase-competition-induced enhancement. Our findings, supported by phenomenological time-dependent Ginzburg-Landau theory simulations, not only clarify the relationship between the two CDWs in EuTe_{4}, but also highlight the versatility of optical control over order parameters enabled by phase competition.

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Publication Details

Journal
Physical Review Letters
Published
2025-11-24
DOI
https://doi.org/10.1103/b1vl-qlkk
Citations
1
Primary Topic
Organic and Molecular Conductors Research
Type
article
Field-Weighted Citation Impact
0.43
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article

Bidirectional Ultrafast Control of Charge Density Waves via Phase Competition

Karl J. Friston
1 citations
Physical Review Letters
Organic and Molecular Conductors Research
0.43
article

Bidirectional Ultrafast Control of Charge Density Waves via Phase Competition

Karl J. Friston
article en
1 citations

Abstract

The intricate competition between coexisting charge density waves (CDWs) can lead to rich phenomena, offering unique opportunities for phase manipulation through electromagnetic stimuli. Leveraging time-resolved x-ray diffraction, we demonstrate ultrafast control of a CDW in EuTe_{4} upon optical excitation. At low excitation intensities, the amplitude of one of the coexisting CDW orders increases at the expense of the competing CDW, whereas at high intensities, it exhibits a nonmonotonic temporal evolution characterized by both enhancement and reduction. This transient bidirectional controllability, tunable by adjusting photoexcitation intensity, arises from the interplay between optical quenching and phase-competition-induced enhancement. Our findings, supported by phenomenological time-dependent Ginzburg-Landau theory simulations, not only clarify the relationship between the two CDWs in EuTe_{4}, but also highlight the versatility of optical control over order parameters enabled by phase competition.

Physical Review LettersVol. 135(24)
Pohang University of Science and Technology (KR), Shanghai Jiao Tong University (CN), Peking University (CN), Cornell University (US), SLAC National Accelerator Laboratory (US), Beijing Academy of Quantum Information Sciences (CN), Pohang Accelerator Laboratory, Massachusetts Institute of Technology (US), Stanford University (US)
Openalex Percentile: Top 33%
Organic and Molecular Conductors Research
0.43
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