X-Ray-Induced Quenching of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mmultiscripts> <mml:mrow> <mml:mi>Th</mml:mi> </mml:mrow> <mml:mprescripts/> <mml:none/> <mml:mrow> <mml:mn>229</mml:mn> </mml:m

Recent studies have shown that the lifetime of the isomeric ^{229}Th doped in crystals can be shortened by x-ray or laser irradiation, a phenomenon referred to as isomer quenching. We investigate the temperature dependence of x-ray-induced quenching in ^{229}Th:CaF_{2} and identify a correlation with the afterglow of the host crystal. These results suggest a mechanism in which x-ray-induced electrons migrate through the lattice and are captured at Th sites, enabling isomer deexcitation via internal conversion through electron-nucleus coupling. This mechanism links nuclear decay to charge carrier dynamics in the host crystal, providing a new interface between nuclear and solid-state physics. The findings offer a pathway to optimize the performance of solid-state nuclear clocks.

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Publication Details

Journal
Physical Review Letters
Published
2025-10-27
DOI
https://doi.org/10.1103/75bb-thn7
Citations
1
Primary Topic
Advanced Frequency and Time Standards
Type
article
Field-Weighted Citation Impact
1.25
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article

X-Ray-Induced Quenching of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mmultiscripts> <mml:mrow> <mml:mi>Th</mml:mi> </mml:mrow> <mml:mprescripts/> <mml:none/> <mml:mrow> <mml:mn>229</mml:mn> </mml:m

Karl J. Friston
1 citations
Physical Review Letters
Advanced Frequency and Time Standards
1.25
article

X-Ray-Induced Quenching of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mmultiscripts> <mml:mrow> <mml:mi>Th</mml:mi> </mml:mrow> <mml:mprescripts/> <mml:none/> <mml:mrow> <mml:mn>229</mml:mn> </mml:m

Karl J. Friston
article en
1 citations

Abstract

Recent studies have shown that the lifetime of the isomeric ^{229}Th doped in crystals can be shortened by x-ray or laser irradiation, a phenomenon referred to as isomer quenching. We investigate the temperature dependence of x-ray-induced quenching in ^{229}Th:CaF_{2} and identify a correlation with the afterglow of the host crystal. These results suggest a mechanism in which x-ray-induced electrons migrate through the lattice and are captured at Th sites, enabling isomer deexcitation via internal conversion through electron-nucleus coupling. This mechanism links nuclear decay to charge carrier dynamics in the host crystal, providing a new interface between nuclear and solid-state physics. The findings offer a pathway to optimize the performance of solid-state nuclear clocks.

Physical Review LettersVol. 136(1)
TU Wien (AT), Kyoto University (JP), SPring-8 (JP), RIKEN (JP), Japan Synchrotron Radiation Research Institute (JP), National Institute of Advanced Industrial Science and Technology (JP)
Openalex Percentile: Top 15%
Advanced Frequency and Time Standards
1.25
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X-Ray-Induced Quenching of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mmultiscripts> <mml:mrow> <mml:mi>Th</mml:mi> </mml:mrow> <mml:mprescripts/> <mml:none/> <mml:mrow> <mml:mn>229</mml:mn> </mml:m — Karl J. Friston · Physical Review Letters (2025) | TGRS Research Map | TGRS