X-Ray-Induced Quenching of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mmultiscripts> <mml:mrow> <mml:mi>Th</mml:mi> </mml:mrow> <mml:mprescripts/> <mml:none/> <mml:mrow> <mml:mn>229</mml:mn> </mml:m
Recent studies have shown that the lifetime of the isomeric ^{229}Th doped in crystals can be shortened by x-ray or laser irradiation, a phenomenon referred to as isomer quenching. We investigate the temperature dependence of x-ray-induced quenching in ^{229}Th:CaF_{2} and identify a correlation with the afterglow of the host crystal. These results suggest a mechanism in which x-ray-induced electrons migrate through the lattice and are captured at Th sites, enabling isomer deexcitation via internal conversion through electron-nucleus coupling. This mechanism links nuclear decay to charge carrier dynamics in the host crystal, providing a new interface between nuclear and solid-state physics. The findings offer a pathway to optimize the performance of solid-state nuclear clocks.
Authors
- Karl J. Friston
Institutions
- TU Wien (AT)
- Kyoto University (JP)
- SPring-8 (JP)
- RIKEN (JP)
- Japan Synchrotron Radiation Research Institute (JP)
- National Institute of Advanced Industrial Science and Technology (JP)
Publication Details
- Journal
- Physical Review Letters
- Published
- 2025-10-27
- DOI
- https://doi.org/10.1103/75bb-thn7
- Citations
- 1
- Primary Topic
- Advanced Frequency and Time Standards
- Type
- article
- Field-Weighted Citation Impact
- 1.25