Incomplete softening of the antiferromagnetic resonance mode at the spin-reorientation transition in multiferroic <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:mi>GdF</mml:mi> <mml:msub> <mml:mi mathvariant="normal">e</mml
The multiferroic ferroborate $\mathrm{GdF}{\mathrm{e}}_{3}{(\mathrm{B}{\mathrm{O}}_{3})}_{4}$ with huntite-type structure exhibits magnetic ordering below ${T}_{\mathrm{N}}=38$ K and contains two magnetic subsystems associated with Gd and Fe ions. Competing anisotropies of these subsystems drive a spin-reorientation transition at ${T}_{\mathrm{SR}}=10.7$ K, switching the ground state from easy-axis to easy-plane. Using antiferromagnetic resonance, we investigate the spin dynamics across this transition. The observed incomplete softening of a magnon mode during both field- and temperature-induced spin-reorientation transitions indicates the first-order nature of the phase transition, which is accompanied by a discontinuous jump in the effective anisotropy field. We reproduce this behavior using a simple model that attributes the jump in the anisotropy field to the presence of an effective fourth-order anisotropy constant, responsible for the discontinuous character of the transition. Remarkably, for in-plane magnetic fields, we identify a new AFMR mode that persists from 12 K up to ${T}_{\mathrm{N}}$. This mode likely corresponds to the dynamics of a long-period incommensurate state, previously detected by resonant elastic x-ray scattering.
Authors
- Veronika Titova (ORCID: https://orcid.org/0000-0003-4390-2971)
- С. Е. Никитин (ORCID: https://orcid.org/0000-0001-8495-1038)
- S. A. Skorobogatov (ORCID: https://orcid.org/0000-0002-4065-8208)
- A. I. Pankrats (ORCID: https://orcid.org/0000-0002-8314-192X)
- И. А. Гудим (ORCID: https://orcid.org/0000-0003-2653-8434)
- I. N. Khoroshiy (ORCID: https://orcid.org/0009-0007-6116-1907)
Institutions
- Russian Academy of Sciences (RU)
- Siberian Federal University (RU)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-10
- DOI
- https://doi.org/10.1103/qlq6-b67j
- Primary Topic
- Crystal Structures and Properties
- Type
- article
- Field-Weighted Citation Impact
- 0.00