Polaron-Polariton-Assisted Thermally Activated Superradiance

We predict an anomalous thermally activated superradiance in molecular aggregates within polaritonic environments. In contrast to free space, the collective emission is enhanced when either the exciton-phonon coupling or the temperature increases. This counterintuitive phenomenon is captured by a microscopic theory that combines macroscopic quantum electrodynamics with a modified polaron quantum master equation approach, revealing a nontrivial interplay among excitons, phonons, and polaritons.

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Publication Details

Journal
Physical Review Letters
Published
2026-06-09
DOI
https://doi.org/10.1103/hs3s-j4yp
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
0.00

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article

Polaron-Polariton-Assisted Thermally Activated Superradiance

Yi-Ting Chuang, Liang‐Yan Hsu
Physical Review Letters
Strong Light-Matter Interactions
article

Polaron-Polariton-Assisted Thermally Activated Superradiance

Yi-Ting Chuang, Liang‐Yan Hsu
article en

Abstract

We predict an anomalous thermally activated superradiance in molecular aggregates within polaritonic environments. In contrast to free space, the collective emission is enhanced when either the exciton-phonon coupling or the temperature increases. This counterintuitive phenomenon is captured by a microscopic theory that combines macroscopic quantum electrodynamics with a modified polaron quantum master equation approach, revealing a nontrivial interplay among excitons, phonons, and polaritons.

Physical Review LettersVol. 136(23)
National Taiwan University (TW), National Center for Theoretical Sciences (TW), National Center for Theoretical Sciences, Physics Division
National Science and Technology Council, National Center for Theoretical Sciences, Academia Sinica, National Science and Technology Council, Physics Division, National Center for Theoretical Sciences
Openalex Percentile: Top 97%
Strong Light-Matter Interactions
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