Nontrivial critical behavior at magnetic transitions: A case study of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>7</mml:mn> </mml:msub> <mml:msub> <mml:mi>Pd</mml:mi> <mml:mn>3</mml:mn>

We present a comprehensive analysis of the critical behavior of ${\mathrm{Sm}}_{7}{\mathrm{Pd}}_{3}$ in the vicinity of its second-order magnetoelastic transition at ${T}_{\mathrm{c}}=173\phantom{\rule{0.16em}{0ex}}\mathrm{K}$. The critical exponents (CEs) $\ensuremath{\beta}$ and $\ensuremath{\gamma}$, determined using both the standard convergence procedure and the average normalized slope (ANS) method, diverge at ${T}_{\mathrm{c}}$---a characteristic typically associated with first-order transitions. Notably, none of the established universality classes satisfactorily describe the critical behavior of ${\mathrm{Sm}}_{7}{\mathrm{Pd}}_{3}$, and we discuss the possible origins of this deviation in the context of the strong spin-lattice coupling intrinsic to the sample. We emphasize the importance of accurately selecting the critical temperature and magnetic field ranges to ensure robust critical behavior analysis, and propose a quantitative approach to assess the reliability of the extracted CEs. Additionally, we demonstrate that in the ANS method, the critical exponents $\ensuremath{\beta}$ and $\ensuremath{\gamma}$ should be calculated separately using data for $T\ensuremath{\leqslant}{T}_{\mathrm{c}}$ and $T\ensuremath{\geqslant}{T}_{\mathrm{c}}$, respectively. Our findings underscore the need for a revised theoretical framework to accurately describe second-order magnetoelastic transitions.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-21
DOI
https://doi.org/10.1103/px6g-hprm
Citations
1
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
1.26
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article

Nontrivial critical behavior at magnetic transitions: A case study of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>7</mml:mn> </mml:msub> <mml:msub> <mml:mi>Pd</mml:mi> <mml:mn>3</mml:mn>

Yaroslav Mudryk, Anis Biswas, Ajay Kumar
1 citations
Physical review. B./Physical review. B
Rare-earth and actinide compounds
1.26
article

Nontrivial critical behavior at magnetic transitions: A case study of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>7</mml:mn> </mml:msub> <mml:msub> <mml:mi>Pd</mml:mi> <mml:mn>3</mml:mn>

Yaroslav Mudryk, Anis Biswas, Ajay Kumar
article en
1 citations

Abstract

We present a comprehensive analysis of the critical behavior of ${\mathrm{Sm}}_{7}{\mathrm{Pd}}_{3}$ in the vicinity of its second-order magnetoelastic transition at ${T}_{\mathrm{c}}=173\phantom{\rule{0.16em}{0ex}}\mathrm{K}$. The critical exponents (CEs) $\ensuremath{\beta}$ and $\ensuremath{\gamma}$, determined using both the standard convergence procedure and the average normalized slope (ANS) method, diverge at ${T}_{\mathrm{c}}$---a characteristic typically associated with first-order transitions. Notably, none of the established universality classes satisfactorily describe the critical behavior of ${\mathrm{Sm}}_{7}{\mathrm{Pd}}_{3}$, and we discuss the possible origins of this deviation in the context of the strong spin-lattice coupling intrinsic to the sample. We emphasize the importance of accurately selecting the critical temperature and magnetic field ranges to ensure robust critical behavior analysis, and propose a quantitative approach to assess the reliability of the extracted CEs. Additionally, we demonstrate that in the ANS method, the critical exponents $\ensuremath{\beta}$ and $\ensuremath{\gamma}$ should be calculated separately using data for $T\ensuremath{\leqslant}{T}_{\mathrm{c}}$ and $T\ensuremath{\geqslant}{T}_{\mathrm{c}}$, respectively. Our findings underscore the need for a revised theoretical framework to accurately describe second-order magnetoelastic transitions.

Physical review. B./Physical review. BVol. 112(22)
Iowa State University (US), Ames National Laboratory (US)
Openalex Percentile: Top 15%
Rare-earth and actinide compounds
1.26
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Nontrivial critical behavior at magnetic transitions: A case study of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>7</mml:mn> </mml:msub> <mml:msub> <mml:mi>Pd</mml:mi> <mml:mn>3</mml:mn> — Yaroslav Mudryk, Anis Biswas, et al. · Physical review. B./Physical review. B (2025) | TGRS Research Map | TGRS