Nontrivial critical behavior at magnetic transitions: A case study of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>7</mml:mn> </mml:msub> <mml:msub> <mml:mi>Pd</mml:mi> <mml:mn>3</mml:mn>
We present a comprehensive analysis of the critical behavior of ${\mathrm{Sm}}_{7}{\mathrm{Pd}}_{3}$ in the vicinity of its second-order magnetoelastic transition at ${T}_{\mathrm{c}}=173\phantom{\rule{0.16em}{0ex}}\mathrm{K}$. The critical exponents (CEs) $\ensuremath{\beta}$ and $\ensuremath{\gamma}$, determined using both the standard convergence procedure and the average normalized slope (ANS) method, diverge at ${T}_{\mathrm{c}}$---a characteristic typically associated with first-order transitions. Notably, none of the established universality classes satisfactorily describe the critical behavior of ${\mathrm{Sm}}_{7}{\mathrm{Pd}}_{3}$, and we discuss the possible origins of this deviation in the context of the strong spin-lattice coupling intrinsic to the sample. We emphasize the importance of accurately selecting the critical temperature and magnetic field ranges to ensure robust critical behavior analysis, and propose a quantitative approach to assess the reliability of the extracted CEs. Additionally, we demonstrate that in the ANS method, the critical exponents $\ensuremath{\beta}$ and $\ensuremath{\gamma}$ should be calculated separately using data for $T\ensuremath{\leqslant}{T}_{\mathrm{c}}$ and $T\ensuremath{\geqslant}{T}_{\mathrm{c}}$, respectively. Our findings underscore the need for a revised theoretical framework to accurately describe second-order magnetoelastic transitions.
Authors
- Yaroslav Mudryk (ORCID: https://orcid.org/0000-0003-2658-0413)
- Anis Biswas (ORCID: https://orcid.org/0000-0003-1733-3082)
- Ajay Kumar (ORCID: https://orcid.org/0000-0002-0840-7951)
Institutions
- Iowa State University (US)
- Ames National Laboratory (US)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-21
- DOI
- https://doi.org/10.1103/px6g-hprm
- Citations
- 1
- Primary Topic
- Rare-earth and actinide compounds
- Type
- article
- Field-Weighted Citation Impact
- 1.26