A quieter state of charge and ultra-low-noise of the collective current in quasi-1D charge-density-wave nanowires

Electronic flicker noise limits phase stability in communication systems, reduces the sensitivity and selectivity of sensors, and degrades coherence in quantum devices. There is a strong need for unconventional materials and strategies for achieving ultra-low-noise performance in nanoscale and quantum electronics. Here, we demonstrate that in nanowires of the quasi-one-dimensional, fully gapped charge-density-wave material (TaSe<sub>4</sub>)<sub>2</sub>I, low-frequency electronic noise is suppressed below the limit of thermalized charge carriers in passive resistors. When the current is dominated by the sliding Frohlich condensate, the normalized noise spectral density, <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub><mml:mrow><mml:mi>S</mml:mi></mml:mrow> <mml:mrow><mml:mi>I</mml:mi></mml:mrow> </mml:msub> <mml:mo>/</mml:mo> <mml:msup><mml:mrow><mml:mi>I</mml:mi></mml:mrow> <mml:mrow><mml:mn>2</mml:mn></mml:mrow> </mml:msup> </mml:math> , decreases linearly with current, <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>I</mml:mi></mml:math> - a striking departure from the constant value of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub><mml:mrow><mml:mi>S</mml:mi></mml:mrow> <mml:mrow><mml:mi>I</mml:mi></mml:mrow> </mml:msub> <mml:mo>/</mml:mo> <mml:msup><mml:mrow><mml:mi>I</mml:mi></mml:mrow> <mml:mrow><mml:mn>2</mml:mn></mml:mrow> </mml:msup> </mml:math> , observed in conventional conductors. No residual minimum noise level is reached for the current of the electron-lattice condensate in (TaSe<sub>4</sub>)<sub>2</sub>I nanowires. Repeating the measurements for another charge-density wave conductor, NbS<sub>3</sub>-II, we found a similar reduction below the normal electron limit at room temperature. Our findings signal intrinsically lower current fluctuations within a correlated electron transport regime.

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Journal
Nature Communications
Published
2025-12-31
DOI
https://doi.org/10.1038/s41467-025-67567-x
Primary Topic
2D Materials and Applications
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article
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article

A quieter state of charge and ultra-low-noise of the collective current in quasi-1D charge-density-wave nanowires

Sergey Rumyantsev, Tina T. Salguero, Nicholas Sesing, Subhajit Ghosh et al.
Nature Communications
2D Materials and Applications
article

A quieter state of charge and ultra-low-noise of the collective current in quasi-1D charge-density-wave nanowires

Sergey Rumyantsev, Tina T. Salguero, Nicholas Sesing, Subhajit Ghosh, Alexander A. Balandin, Roger K. Lake
article en

Abstract

Electronic flicker noise limits phase stability in communication systems, reduces the sensitivity and selectivity of sensors, and degrades coherence in quantum devices. There is a strong need for unconventional materials and strategies for achieving ultra-low-noise performance in nanoscale and quantum electronics. Here, we demonstrate that in nanowires of the quasi-one-dimensional, fully gapped charge-density-wave material (TaSe<sub>4</sub>)<sub>2</sub>I, low-frequency electronic noise is suppressed below the limit of thermalized charge carriers in passive resistors. When the current is dominated by the sliding Frohlich condensate, the normalized noise spectral density, <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub><mml:mrow><mml:mi>S</mml:mi></mml:mrow> <mml:mrow><mml:mi>I</mml:mi></mml:mrow> </mml:msub> <mml:mo>/</mml:mo> <mml:msup><mml:mrow><mml:mi>I</mml:mi></mml:mrow> <mml:mrow><mml:mn>2</mml:mn></mml:mrow> </mml:msup> </mml:math> , decreases linearly with current, <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>I</mml:mi></mml:math> - a striking departure from the constant value of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub><mml:mrow><mml:mi>S</mml:mi></mml:mrow> <mml:mrow><mml:mi>I</mml:mi></mml:mrow> </mml:msub> <mml:mo>/</mml:mo> <mml:msup><mml:mrow><mml:mi>I</mml:mi></mml:mrow> <mml:mrow><mml:mn>2</mml:mn></mml:mrow> </mml:msup> </mml:math> , observed in conventional conductors. No residual minimum noise level is reached for the current of the electron-lattice condensate in (TaSe<sub>4</sub>)<sub>2</sub>I nanowires. Repeating the measurements for another charge-density wave conductor, NbS<sub>3</sub>-II, we found a similar reduction below the normal electron limit at room temperature. Our findings signal intrinsically lower current fluctuations within a correlated electron transport regime.

Nature CommunicationsVol. 17(1)
University of California, Riverside (US), California NanoSystems Institute (US), University of California, Los Angeles (US), University of Georgia (US), Institute of High Pressure Physics (PL), Polish Academy of Sciences (PL)
National Institutes of Health, Office of Naval Research, California NanoSystems Institute
Openalex Percentile: Top 68%
2D Materials and Applications
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