Dominant Kitaev interaction and field-induced quantum disordered phase in the cobaltate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Na</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>Co</mml:mi>

The identification of quantum spin-liquid phases in Kitaev candidate materials remains a major experimental challenge. Since most Kitaev candidates develop antiferromagnetic (AFM) order at low temperatures, currently there is great interest on the field-induced magnetic disordered phase in these compounds that are distinct from (partially) polarized states. Recently, a cobaltate ${\mathrm{Na}}_{2}{\mathrm{Co}}_{2}{\mathrm{TeO}}_{6}$ has emerged as a promising Kitaev candidate with high-spin ${t}_{2g}^{5}{e}_{g}^{2}$ configuration and spin-orbit-entangled ${J}_{\mathrm{eff}}=1/2$ honeycomb lattice system. There are intensive studies on field-induced magnetic states and phase transitions under in-plane magnetic fields. In this study, we propose an intermediate disordered phase induced by an out-of-plane field along the $c$-axis, through high-field magnetization and magnetocaloric effect measurements. To explain the high-field behavior of ${\mathrm{Na}}_{2}{\mathrm{Co}}_{2}{\mathrm{TeO}}_{6}$, we develop an effective $K\text{\ensuremath{-}}J\text{\ensuremath{-}}\mathrm{\ensuremath{\Gamma}}\text{\ensuremath{-}}{\mathrm{\ensuremath{\Gamma}}}^{\ensuremath{'}}$ spin model featuring a dominant AFM Kitaev interaction. This framework uncovers an intermediate quantum spin-liquid phase, establishing the material as a unique platform for exploring Kitaev physics and field-induced quantum-disordered states.

Authors

Institutions

Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-14
DOI
https://doi.org/10.1103/r574-yrrp
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
0.00
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Dominant Kitaev interaction and field-induced quantum disordered phase in the cobaltate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Na</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>Co</mml:mi>

Akira Matsuo, Je‐Geun Park, Gang Su, Koichi Kindo et al.
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
article

Dominant Kitaev interaction and field-induced quantum disordered phase in the cobaltate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Na</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>Co</mml:mi>

Akira Matsuo, Je‐Geun Park, Gang Su, Koichi Kindo, Yoshimitsu Kohama, Zhuo Yang, Kavita Mehlawat, Atsuhiko Miyata, Chaebin Kim, Yasuhiro H. Matsuda, Xu-Guang Zhou, Wei Li, Han Li, Kazuki Matsui
article en

Abstract

The identification of quantum spin-liquid phases in Kitaev candidate materials remains a major experimental challenge. Since most Kitaev candidates develop antiferromagnetic (AFM) order at low temperatures, currently there is great interest on the field-induced magnetic disordered phase in these compounds that are distinct from (partially) polarized states. Recently, a cobaltate ${\mathrm{Na}}_{2}{\mathrm{Co}}_{2}{\mathrm{TeO}}_{6}$ has emerged as a promising Kitaev candidate with high-spin ${t}_{2g}^{5}{e}_{g}^{2}$ configuration and spin-orbit-entangled ${J}_{\mathrm{eff}}=1/2$ honeycomb lattice system. There are intensive studies on field-induced magnetic states and phase transitions under in-plane magnetic fields. In this study, we propose an intermediate disordered phase induced by an out-of-plane field along the $c$-axis, through high-field magnetization and magnetocaloric effect measurements. To explain the high-field behavior of ${\mathrm{Na}}_{2}{\mathrm{Co}}_{2}{\mathrm{TeO}}_{6}$, we develop an effective $K\text{\ensuremath{-}}J\text{\ensuremath{-}}\mathrm{\ensuremath{\Gamma}}\text{\ensuremath{-}}{\mathrm{\ensuremath{\Gamma}}}^{\ensuremath{'}}$ spin model featuring a dominant AFM Kitaev interaction. This framework uncovers an intermediate quantum spin-liquid phase, establishing the material as a unique platform for exploring Kitaev physics and field-induced quantum-disordered states.

Physical review. B./Physical review. BVol. 112(24)
Georgia Institute of Technology (US), Seoul National University (KR), Chinese Academy of Sciences (CN), Beijing Jiaotong University (CN), University of Chinese Academy of Sciences (CN), The University of Tokyo (JP)
Openalex Percentile: Top 75%
Advanced Condensed Matter Physics
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.