Dominant Kitaev interaction and field-induced quantum disordered phase in the cobaltate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Na</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>Co</mml:mi>
The identification of quantum spin-liquid phases in Kitaev candidate materials remains a major experimental challenge. Since most Kitaev candidates develop antiferromagnetic (AFM) order at low temperatures, currently there is great interest on the field-induced magnetic disordered phase in these compounds that are distinct from (partially) polarized states. Recently, a cobaltate ${\mathrm{Na}}_{2}{\mathrm{Co}}_{2}{\mathrm{TeO}}_{6}$ has emerged as a promising Kitaev candidate with high-spin ${t}_{2g}^{5}{e}_{g}^{2}$ configuration and spin-orbit-entangled ${J}_{\mathrm{eff}}=1/2$ honeycomb lattice system. There are intensive studies on field-induced magnetic states and phase transitions under in-plane magnetic fields. In this study, we propose an intermediate disordered phase induced by an out-of-plane field along the $c$-axis, through high-field magnetization and magnetocaloric effect measurements. To explain the high-field behavior of ${\mathrm{Na}}_{2}{\mathrm{Co}}_{2}{\mathrm{TeO}}_{6}$, we develop an effective $K\text{\ensuremath{-}}J\text{\ensuremath{-}}\mathrm{\ensuremath{\Gamma}}\text{\ensuremath{-}}{\mathrm{\ensuremath{\Gamma}}}^{\ensuremath{'}}$ spin model featuring a dominant AFM Kitaev interaction. This framework uncovers an intermediate quantum spin-liquid phase, establishing the material as a unique platform for exploring Kitaev physics and field-induced quantum-disordered states.
Authors
- Akira Matsuo
- Je‐Geun Park (ORCID: https://orcid.org/0000-0002-3930-4226)
- Gang Su (ORCID: https://orcid.org/0000-0002-8149-4342)
- Koichi Kindo
- Yoshimitsu Kohama (ORCID: https://orcid.org/0000-0003-0149-704X)
- Zhuo Yang (ORCID: https://orcid.org/0000-0003-4727-7907)
- Kavita Mehlawat (ORCID: https://orcid.org/0000-0001-9603-2688)
- Atsuhiko Miyata (ORCID: https://orcid.org/0000-0002-1726-0314)
- Chaebin Kim (ORCID: https://orcid.org/0000-0001-5392-7756)
- Yasuhiro H. Matsuda (ORCID: https://orcid.org/0000-0002-7450-0791)
- Xu-Guang Zhou (ORCID: https://orcid.org/0000-0001-9081-5243)
- Wei Li (ORCID: https://orcid.org/0000-0003-0474-9337)
- Han Li (ORCID: https://orcid.org/0000-0003-0071-8461)
- Kazuki Matsui (ORCID: https://orcid.org/0009-0005-6032-0828)
Institutions
- Georgia Institute of Technology (US)
- Seoul National University (KR)
- Chinese Academy of Sciences (CN)
- Beijing Jiaotong University (CN)
- University of Chinese Academy of Sciences (CN)
- The University of Tokyo (JP)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-14
- DOI
- https://doi.org/10.1103/r574-yrrp
- Primary Topic
- Advanced Condensed Matter Physics
- Type
- article
- Field-Weighted Citation Impact
- 0.00