Short-range spin freezing in the double trillium lattice spin-liquid candidate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>KSrFe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mrow> <mml:mo>(</mml:

The authors investigate here the double-trillium lattice antiferromagnet KSrFe${}_{2}$(PO${}_{4}$)${}_{3}$ using ${}^{31}$P NMR, thermodynamic measurements, and first-principles calculations to elucidate its unconventional ground state. Below the characteristic temperature $T$* ~ 3.5 K, the results reveal a short-range spin freezing state with persistent antiferromagnetic fluctuations, contradicting earlier proposals of a gapless spin-liquid state. A nearly field-independent NMR linewidth, strong enhancement of 1/${T}_{2}$ below $T$*, and sizeable antiferromagnetic exchange interactions collectively position KSrFe${}_{2}$(PO${}_{4}$)${}_{3}$ as a rare three-dimensional frustrated magnet hosting intertwined static and dynamic correlations.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-14
DOI
https://doi.org/10.1103/k3lw-2567
Citations
1
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
1.26
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article

Short-range spin freezing in the double trillium lattice spin-liquid candidate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>KSrFe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mrow> <mml:mo>(</mml:

Alexander A. Tsirlin, Sebin J. Sebastian, Qing-Ping Ding, R. Nath et al.
1 citations
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
1.26
article

Short-range spin freezing in the double trillium lattice spin-liquid candidate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>KSrFe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mrow> <mml:mo>(</mml:

Alexander A. Tsirlin, Sebin J. Sebastian, Qing-Ping Ding, R. Nath, Yuji Furukawa
article en
1 citations

Abstract

The authors investigate here the double-trillium lattice antiferromagnet KSrFe${}_{2}$(PO${}_{4}$)${}_{3}$ using ${}^{31}$P NMR, thermodynamic measurements, and first-principles calculations to elucidate its unconventional ground state. Below the characteristic temperature $T$* ~ 3.5 K, the results reveal a short-range spin freezing state with persistent antiferromagnetic fluctuations, contradicting earlier proposals of a gapless spin-liquid state. A nearly field-independent NMR linewidth, strong enhancement of 1/${T}_{2}$ below $T$*, and sizeable antiferromagnetic exchange interactions collectively position KSrFe${}_{2}$(PO${}_{4}$)${}_{3}$ as a rare three-dimensional frustrated magnet hosting intertwined static and dynamic correlations.

Physical review. B./Physical review. BVol. 112(22)
Iowa State University (US), Ames National Laboratory (US), Leipzig University (DE)
Openalex Percentile: Top 15%
Advanced Condensed Matter Physics
1.26
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