Short-range spin freezing in the double trillium lattice spin-liquid candidate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>KSrFe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mrow> <mml:mo>(</mml:
The authors investigate here the double-trillium lattice antiferromagnet KSrFe${}_{2}$(PO${}_{4}$)${}_{3}$ using ${}^{31}$P NMR, thermodynamic measurements, and first-principles calculations to elucidate its unconventional ground state. Below the characteristic temperature $T$* ~ 3.5 K, the results reveal a short-range spin freezing state with persistent antiferromagnetic fluctuations, contradicting earlier proposals of a gapless spin-liquid state. A nearly field-independent NMR linewidth, strong enhancement of 1/${T}_{2}$ below $T$*, and sizeable antiferromagnetic exchange interactions collectively position KSrFe${}_{2}$(PO${}_{4}$)${}_{3}$ as a rare three-dimensional frustrated magnet hosting intertwined static and dynamic correlations.
Authors
- Alexander A. Tsirlin (ORCID: https://orcid.org/0000-0001-6916-8256)
- Sebin J. Sebastian (ORCID: https://orcid.org/0000-0002-0184-0787)
- Qing-Ping Ding (ORCID: https://orcid.org/0000-0001-7488-066X)
- R. Nath (ORCID: https://orcid.org/0000-0003-1613-3652)
- Yuji Furukawa (ORCID: https://orcid.org/0000-0002-3722-293X)
Institutions
- Iowa State University (US)
- Ames National Laboratory (US)
- Leipzig University (DE)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-14
- DOI
- https://doi.org/10.1103/k3lw-2567
- Citations
- 1
- Primary Topic
- Advanced Condensed Matter Physics
- Type
- article
- Field-Weighted Citation Impact
- 1.26