Stability of algebraic spin liquids coupled to quantum phonons

Algebraic spin liquids are quantum disordered phases of insulating magnets that exhibit fractionalized gapless excitations and power-law correlations. Quantum spin liquids in this category include the experimentally established one-dimensional (1D) Luttinger liquid, as well as the U(1) Dirac spin liquid (DSL) that has been a focus of recent candidate materials searches. Most notably, several exchange-frustrated Heisenberg materials on the triangular lattice have shown evidence of the U(1) DSL. In this work, we measure the algebraic correlations of spin-singlet excitations in the <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi>J</a:mi> <a:mn>1</a:mn> </a:msub> <a:mtext>−</a:mtext> <a:msub> <a:mi>J</a:mi> <a:mn>2</a:mn> </a:msub> </a:mrow> </a:math> antiferromagnetic Heisenberg model on the triangular lattice, prompting a detailed investigation of this model’s stability under spin-lattice coupling with dynamical phonons using variational Monte Carlo. As seen before in 1D spin chains, we observe a low-temperature transition from a U(1) DSL to valence bond order and predict the parameter regime where the model realizes a stable DSL ground state. To achieve this, we employ a series of finite-size scaling Ansätze inspired by the low-energy DSL’s conformal description in terms of quantum electrodynamics and show that emergent monopole operators drive the instability. We compare the physics of this transition to the 1D Luttinger liquid throughout our analysis. We derive the regime of stability against spin-Peierls ordering and argue that the DSL ground state might still be achievable in candidate materials, despite its tendency to valence bond solid ordering.

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Journal
Physical Review Research
Published
2025-11-16
DOI
https://doi.org/10.1103/9wnn-w8bg
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
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article

Stability of algebraic spin liquids coupled to quantum phonons

Johannes Knolle, Urban F. P. Seifert, Francesco Ferrari, Roser Valentí et al.
Physical Review Research
Advanced Condensed Matter Physics
article

Stability of algebraic spin liquids coupled to quantum phonons

Johannes Knolle, Urban F. P. Seifert, Francesco Ferrari, Roser Valentí, Josef Willsher
article en

Abstract

Algebraic spin liquids are quantum disordered phases of insulating magnets that exhibit fractionalized gapless excitations and power-law correlations. Quantum spin liquids in this category include the experimentally established one-dimensional (1D) Luttinger liquid, as well as the U(1) Dirac spin liquid (DSL) that has been a focus of recent candidate materials searches. Most notably, several exchange-frustrated Heisenberg materials on the triangular lattice have shown evidence of the U(1) DSL. In this work, we measure the algebraic correlations of spin-singlet excitations in the <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi>J</a:mi> <a:mn>1</a:mn> </a:msub> <a:mtext>−</a:mtext> <a:msub> <a:mi>J</a:mi> <a:mn>2</a:mn> </a:msub> </a:mrow> </a:math> antiferromagnetic Heisenberg model on the triangular lattice, prompting a detailed investigation of this model’s stability under spin-lattice coupling with dynamical phonons using variational Monte Carlo. As seen before in 1D spin chains, we observe a low-temperature transition from a U(1) DSL to valence bond order and predict the parameter regime where the model realizes a stable DSL ground state. To achieve this, we employ a series of finite-size scaling Ansätze inspired by the low-energy DSL’s conformal description in terms of quantum electrodynamics and show that emergent monopole operators drive the instability. We compare the physics of this transition to the 1D Luttinger liquid throughout our analysis. We derive the regime of stability against spin-Peierls ordering and argue that the DSL ground state might still be achievable in candidate materials, despite its tendency to valence bond solid ordering.

Physical Review ResearchVol. 7(4)
Kavli Institute for Theoretical Sciences (CN), Max Planck Institute for the Physics of Complex Systems (DE), Instituto de Física Teórica (ES), Munich Center for Quantum Science and Technology (DE), Imperial College London (GB), Technical University of Munich (DE)
Openalex Percentile: Top 75%
Advanced Condensed Matter Physics
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