Evidence of an exchange-based origin of demagnetization from the fluence dependent delay of Ni in a disordered <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Fe</mml:mi> <mml:mrow> <mml:mn>0.5</mml:mn> </mml:m

The delayed demagnetization in Ni relative to Fe in the ultrafast demagnetization studies in FeNi alloy has led to two competing theoretical explanations: The Inhomogeneous Magnon Generation (IMG) and the Optically Induced Spin Transfer (OISTR) model. The IMG attributes the delay to the preferential magnon generation at the Fe sites and its subsequent propagation to Ni, while OISTR proposes direct spin transfer from Ni to Fe. In this study, we employ element-resolved extreme ultraviolet spectroscopy to investigate the effect of excitation strength on this delay, aiming to resolve the controversy. The data indicate a significant reduction in the delay with increasing fluence, which is inconsistent with the theoretical predictions of OISTR. These findings, in conjunction with the observation of a saturation of Fe demagnetization at the onset of Ni demagnetization, indicate that a spin-wave instability within the IMG framework may provide a potential explanation for the experimental results.

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Journal
Physical review. B./Physical review. B
Published
2025-10-31
DOI
https://doi.org/10.1103/f39s-kvy8
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
0.00

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article

Evidence of an exchange-based origin of demagnetization from the fluence dependent delay of Ni in a disordered <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Fe</mml:mi> <mml:mrow> <mml:mn>0.5</mml:mn> </mml:m

Clemens von Korff Schmising, Puloma Singh, Stefan Eisebitt, Olof Karis et al.
Physical review. B./Physical review. B
Magnetic properties of thin films
article

Evidence of an exchange-based origin of demagnetization from the fluence dependent delay of Ni in a disordered <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Fe</mml:mi> <mml:mrow> <mml:mn>0.5</mml:mn> </mml:m

Clemens von Korff Schmising, Puloma Singh, Stefan Eisebitt, Olof Karis, Kelvin Yao, J. Richter, Denny Sommer, Ronny Knut, Somnath Jana, Dieter Engel, Daniel Schick, Christian Tzschaschel
article en

Abstract

The delayed demagnetization in Ni relative to Fe in the ultrafast demagnetization studies in FeNi alloy has led to two competing theoretical explanations: The Inhomogeneous Magnon Generation (IMG) and the Optically Induced Spin Transfer (OISTR) model. The IMG attributes the delay to the preferential magnon generation at the Fe sites and its subsequent propagation to Ni, while OISTR proposes direct spin transfer from Ni to Fe. In this study, we employ element-resolved extreme ultraviolet spectroscopy to investigate the effect of excitation strength on this delay, aiming to resolve the controversy. The data indicate a significant reduction in the delay with increasing fluence, which is inconsistent with the theoretical predictions of OISTR. These findings, in conjunction with the observation of a saturation of Fe demagnetization at the onset of Ni demagnetization, indicate that a spin-wave instability within the IMG framework may provide a potential explanation for the experimental results.

Physical review. B./Physical review. BVol. 112(21)
Uppsala University (SE), Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE), Technische Universität Berlin (DE)
Deutsche Forschungsgemeinschaft, Knut och Alice Wallenbergs Stiftelse, Vetenskapsrådet, Leibniz-Gemeinschaft
Openalex Percentile: Top 69%
Magnetic properties of thin films
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