Interface magnetism and anomalous Hall effect in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi mathvariant="normal">La</mml:mi> <mml:mrow> <mml:mn>0.7</mml:mn> </mml:mrow> </mml:msub> <mml:msub> <mml:mi mathv

Epitaxial interfaces combining 3d and 5d transition metal oxides are a fertile playground to examine the interplay between topology and electron correlations. In this paper, we explore magnetism and transport of bilayers combining ferromagnetic <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi mathvariant="normal">La</a:mi> <a:mrow> <a:mn>0.7</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi mathvariant="normal">Sr</a:mi> <a:mrow> <a:mn>0.3</a:mn> </a:mrow> </a:msub> <a:mi>Mn</a:mi> <a:msub> <a:mi mathvariant="normal">O</a:mi> <a:mn>3</a:mn> </a:msub> </a:mrow> </a:math> and the strong spin-orbit coupling material <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"> <e:mrow> <e:mi>SrIr</e:mi> <e:msub> <e:mi mathvariant="normal">O</e:mi> <e:mn>3</e:mn> </e:msub> </e:mrow> </e:math> . We have found an interfacial magnetic proximity effect driving an intrinsic contribution to the anomalous Hall effect of topological origin. The interfacial proximity interaction is enabled by the Mn-O-Ir bonding reconstruction and depends on layer sequence. While bilayers with the <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"> <g:mrow> <g:msub> <g:mi mathvariant="normal">La</g:mi> <g:mrow> <g:mn>0.7</g:mn> </g:mrow> </g:msub> <g:msub> <g:mi mathvariant="normal">Sr</g:mi> <g:mrow> <g:mn>0.3</g:mn> </g:mrow> </g:msub> <g:mi>Mn</g:mi> <g:msub> <g:mi mathvariant="normal">O</g:mi> <g:mn>3</g:mn> </g:msub> </g:mrow> </g:math> on top featuring a robust Mn magnetism at the interface show the intrinsic AHE contribution, it is absent in bilayers with the inverted layer sequence ( <k:math xmlns:k="http://www.w3.org/1998/Math/MathML"> <k:mrow> <k:mi>SrIr</k:mi> <k:msub> <k:mi mathvariant="normal">O</k:mi> <k:mn>3</k:mn> </k:msub> </k:mrow> </k:math> layer on top) showing strongly suppressed magnetism at the interface. These results illustrate the leading role of interfacial atomic reconstructions on the interplay between topology and correlations at 3d/5d oxide interfaces. This finding may be of interest in future oxide topological spintronics and spin-orbitronics.

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Journal
Physical Review Materials
Published
2025-12-04
DOI
https://doi.org/10.1103/qxn3-5327
Primary Topic
Magnetic and transport properties of perovskites and related materials
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article
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Interface magnetism and anomalous Hall effect in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi mathvariant="normal">La</mml:mi> <mml:mrow> <mml:mn>0.7</mml:mn> </mml:mrow> </mml:msub> <mml:msub> <mml:mi mathv

Timothy Charlton, Yongseong Choi, J. Tornos, Stephan Rosenkranz et al.
Physical Review Materials
Magnetic and transport properties of perovskites and related materials
article

Interface magnetism and anomalous Hall effect in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi mathvariant="normal">La</mml:mi> <mml:mrow> <mml:mn>0.7</mml:mn> </mml:mrow> </mml:msub> <mml:msub> <mml:mi mathv

Timothy Charlton, Yongseong Choi, J. Tornos, Stephan Rosenkranz, Mariona Cabero, Javier E. Villegas, B. J. Kirby, D. Haskel, Myoung-Woo Yoo, J. Santamarı́a, J.M. González-Calbet, M. Garcı́a-Hernández, F. J. Mompeán, S. G. E. te Velthuis, C. León, Z. Sefrioui, A. Rivera, Sandra Pradana López, Xiao Wang, Joerg Strempfer, Andrea Peralta-Somoza, Rafael Fuster
article en

Abstract

Epitaxial interfaces combining 3d and 5d transition metal oxides are a fertile playground to examine the interplay between topology and electron correlations. In this paper, we explore magnetism and transport of bilayers combining ferromagnetic <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi mathvariant="normal">La</a:mi> <a:mrow> <a:mn>0.7</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi mathvariant="normal">Sr</a:mi> <a:mrow> <a:mn>0.3</a:mn> </a:mrow> </a:msub> <a:mi>Mn</a:mi> <a:msub> <a:mi mathvariant="normal">O</a:mi> <a:mn>3</a:mn> </a:msub> </a:mrow> </a:math> and the strong spin-orbit coupling material <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"> <e:mrow> <e:mi>SrIr</e:mi> <e:msub> <e:mi mathvariant="normal">O</e:mi> <e:mn>3</e:mn> </e:msub> </e:mrow> </e:math> . We have found an interfacial magnetic proximity effect driving an intrinsic contribution to the anomalous Hall effect of topological origin. The interfacial proximity interaction is enabled by the Mn-O-Ir bonding reconstruction and depends on layer sequence. While bilayers with the <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"> <g:mrow> <g:msub> <g:mi mathvariant="normal">La</g:mi> <g:mrow> <g:mn>0.7</g:mn> </g:mrow> </g:msub> <g:msub> <g:mi mathvariant="normal">Sr</g:mi> <g:mrow> <g:mn>0.3</g:mn> </g:mrow> </g:msub> <g:mi>Mn</g:mi> <g:msub> <g:mi mathvariant="normal">O</g:mi> <g:mn>3</g:mn> </g:msub> </g:mrow> </g:math> on top featuring a robust Mn magnetism at the interface show the intrinsic AHE contribution, it is absent in bilayers with the inverted layer sequence ( <k:math xmlns:k="http://www.w3.org/1998/Math/MathML"> <k:mrow> <k:mi>SrIr</k:mi> <k:msub> <k:mi mathvariant="normal">O</k:mi> <k:mn>3</k:mn> </k:msub> </k:mrow> </k:math> layer on top) showing strongly suppressed magnetism at the interface. These results illustrate the leading role of interfacial atomic reconstructions on the interplay between topology and correlations at 3d/5d oxide interfaces. This finding may be of interest in future oxide topological spintronics and spin-orbitronics.

Physical Review MaterialsVol. 9(12)
Bryn Mawr College (US), Universidad Complutense de Madrid (ES), Argonne National Laboratory (US), Oak Ridge National Laboratory (US), National Institute of Standards and Technology (US), University of Illinois Urbana-Champaign (US), International Council on Mining and Metals (GB), Université Paris-Saclay (FR), Instituto de Ciencia de Materiales de Madrid (ES), National Institute of Standards (EG), NIST Center for Neutron Research (US)
Openalex Percentile: Top 72%
Magnetic and transport properties of perovskites and related materials
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