Ultrafast optical evidence of coexisting density waves in bilayer nickelate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>La</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi>Ni</mml:mi> <mml:mn>2</m
Utilizing ultrafast optical pump-probe spectroscopy, we investigate the coexistence and competition of electronic orders in the bilayer nickelate ${\mathrm{La}}_{3}{\mathrm{Ni}}_{2}{\mathrm{O}}_{7}$. Our results reveal two coexisting density waves that can be selectively manipulated with light. We directly identify a spin-density wave (SDW) with electronic nematicity emerging below ${T}_{\mathrm{SDW}}$ $\ensuremath{\approx}140$ K by measuring its spin dynamics, and discover a distinct, nonmagnetic charge order appearing below ${T}_{\mathrm{DW}}$ $\ensuremath{\approx}115$ K. The central finding is the demonstration of differential optical control: the charge order is fragile, completely suppressed by a pump fluence of approximately 40 $\textmu{}\mathrm{J}/{\mathrm{cm}}^{2}$, while the SDW is remarkably robust, persisting to 200 $\textmu{}\mathrm{J}/{\mathrm{cm}}^{2}$. This work establishes a clear hierarchy in the stability of competing electronic orders and provides a powerful method for disentangling their interplay in quantum materials.
Authors
- Jian-Qiao Meng (ORCID: https://orcid.org/0000-0003-3168-9819)
- Yu-Xia Duan (ORCID: https://orcid.org/0000-0002-4581-0686)
- Zijie Xu (ORCID: https://orcid.org/0000-0002-7392-8534)
- Zhanli Fu
- De‐Yuan Hu
- Mengwu Huo (ORCID: https://orcid.org/0009-0007-0530-8310)
- Hai-Long Deng
- Ying Zhou (ORCID: https://orcid.org/0000-0002-1244-3859)
- Jun Liu (ORCID: https://orcid.org/0000-0001-7026-1941)
- Chen Zhang (ORCID: https://orcid.org/0000-0003-3321-4171)
- Meng Wang (ORCID: https://orcid.org/0000-0002-8232-2331)
- Bo Chen (ORCID: https://orcid.org/0000-0002-0404-2799)
- Qi-Yi Wu (ORCID: https://orcid.org/0009-0000-5258-3955)
- Caifeng Lv
- Hao Liu (ORCID: https://orcid.org/0000-0002-2366-9554)
Institutions
- Central South University (CN)
- Beijing Academy of Quantum Information Sciences (CN)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-12
- DOI
- https://doi.org/10.1103/j6hl-t2sh
- Primary Topic
- Magnetic and transport properties of perovskites and related materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00