Projector method for nonlinear light-matter interactions and quantum geometry

We develop a systematic projector-based Feynman diagram framework that intrinsically encodes quantum geometry for nonlinear optical responses. By explicitly incorporating geometric quantities such as the quantum geometric tensor, quantum hermitian connection, and triple-phase product, the method ensures componentwise gauge invariance and seamlessly extends to multiband systems, enabling accurate calculations of quantum geometry and nonlinear optical responses. We derive the projector formalism in the Wannier function basis and implement the ab initio calculations of shift current in GeS, demonstrating excellent agreement with the sum rule and Wilson loop approaches. This work extends projector-based representations within the Wannier functions basis, offering an efficient and reliable tool for investigating nonlinear light-matter interactions and quantum geometry in realistic materials.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-12
DOI
https://doi.org/10.1103/qd9q-hnfp
Primary Topic
Mechanical and Optical Resonators
Type
article
Field-Weighted Citation Impact
0.00
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article

Projector method for nonlinear light-matter interactions and quantum geometry

Zhichao Guo, Hua Wang, Zhuocheng Lu
Physical review. B./Physical review. B
Mechanical and Optical Resonators
article

Projector method for nonlinear light-matter interactions and quantum geometry

Zhichao Guo, Hua Wang, Zhuocheng Lu
article en

Abstract

We develop a systematic projector-based Feynman diagram framework that intrinsically encodes quantum geometry for nonlinear optical responses. By explicitly incorporating geometric quantities such as the quantum geometric tensor, quantum hermitian connection, and triple-phase product, the method ensures componentwise gauge invariance and seamlessly extends to multiband systems, enabling accurate calculations of quantum geometry and nonlinear optical responses. We derive the projector formalism in the Wannier function basis and implement the ab initio calculations of shift current in GeS, demonstrating excellent agreement with the sum rule and Wilson loop approaches. This work extends projector-based representations within the Wannier functions basis, offering an efficient and reliable tool for investigating nonlinear light-matter interactions and quantum geometry in realistic materials.

Physical review. B./Physical review. BVol. 112(23)
Zhejiang Lab (CN), Zhejiang University (CN)
Openalex Percentile: Top 70%
Mechanical and Optical Resonators
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